Sonochemical synthesis and loading of PbS nanoparticles into mesoporous silica

被引：25

作者：

Akbay, Elif ^{[1
]}

Olmez, Tufan Gur ^{[1
]}

机构：

[1] Anadolu Univ, Chem Engn, Eskisehir, Turkey

来源：

MATERIALS LETTERS | 2018年 / 215卷

关键词：

PbS; SBA-15; Sonochemical synthesis; Semiconductor; QUANTUM DOTS; NANOCOMPOSITE; NANOCRYSTALLITES; MORPHOLOGIES; REDUCTION; PROPERTY; NANORODS; ARRAYS;

D O I：

10.1016/j.matlet.2017.12.117

中图分类号：

T [工业技术];

学科分类号：

120111 [工业工程];

摘要：

A sonochemical method was used for simultaneous synthesis and loading of lead sulfide (PbS) nanoparticles into mesoporous SBA-15 (Santa Barbara Amorphous). In this study, the effect of different loading ratios (30, 45, 60, 75%) on morphology, crystalline structure and physicochemical characteristics of PbS-SBA-15_samples was investigated. TEM images showed that the PbS nanoparticles were highly dispersed inside the SBA-15 pores for all tested loadings, however especially 60 and 75%-PbS-SBA15_samples exhibited significant surface aggregation of PbS on SBA-15 surface. Also, PbS-SBA15_samples showed a strong UV light absorption at about 290-310 nm with increasing band gap energies, which is indicative of quantization effects. (C) 2017 Elsevier B.V. All rights reserved.

引用

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页码：263 / 267

页数：5

相关论文

共 27 条

[1]

Effect of Synthesis Conditions on the Structure and Catalytic Performance of V- and Ce-Incorporated SBA-15-like Materials in Propane Selective Oxidation [J].

Aktas, Ozge ;

Yasyerli, Sena ;

Dogu, Gulsen ;

Dogu, Timur .

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2010, 49 (15) :6790-6802

[2]

Citral hydrogenation on high surface area mesoporous TiO2-SiO2 supported Pt nanocomposites: Effect of titanium loading and reduction temperature on the catalytic performances [J].

Bidaoui, Mourad ;

Especel, Catherine ;

Bouchenafa-Saib, Naima ;

Duprez, Daniel ;

Mohammedi, Ourida ;

Royer, Sebastien .

APPLIED CATALYSIS A-GENERAL, 2012, 445 :14-25

[3]

Enhanced visible-light-responsive photocatalytic property of PbS-sensitized K4Nb6O17 nanocomposite photocatalysts [J].

Cui, Wenquan ;

Shao, Meiyi ;

Liu, Li ;

Liang, Yinghua ;

Rana, Dipak .

APPLIED SURFACE SCIENCE, 2013, 276 :823-831

[4]

Selective methane bromination over sulfated zirconia in SBA-15 catalysts [J].

Degirmenci, Volkan ;

Yilmaz, Aysen ;

Uner, Deniz .

CATALYSIS TODAY, 2009, 142 (1-2) :30-33

[5]

Formation, near-infrared luminescence and multi-wavelength optical amplification of PbS quantum dot-embedded silicate glasses [J].

Dong, Guoping ;

Wu, Guobo ;

Fan, Shaohua ;

Zhang, Fangteng ;

Zhang, Yuanhao ;

Wu, Botao ;

Ma, Zhijun ;

Peng, Mingying ;

Qiu, Jianrong .

JOURNAL OF NON-CRYSTALLINE SOLIDS, 2014, 383 :192-195

[6]

Facile synthesis of CuO@PbS core/shell nanowire arrays [J].

Farshidi, Hajar ;

Youzbashi, Amir Ali ;

Saani, Mehdi Heidari ;

Rashidi, Alimorad ;

Kazemzadeh, Asghar ;

Kiani, Fatemeh .

MATERIALS LETTERS, 2017, 193 :259-262

[7]

Controlled synthesis of semiconductor PbS nanocrystals and nanowires inside mesoporous silica SBA-15 phase [J].

Gao, F ;

Lu, QY ;

Liu, XY ;

Yan, YS ;

Zhao, DY .

NANO LETTERS, 2001, 1 (12) :743-748

[8]

A novel method for PbS quantum dot synthesis [J].

Jiao, Yuechao ;

Gao, Xiaoyong ;

Lu, Jingxiao ;

Chen, Yongsheng ;

Zhou, Jianpeng ;

Li, Xinli .

MATERIALS LETTERS, 2012, 72 :116-118

[9]

Ultrasensitive solution-cast quantum dot photodetectors [J].

Konstantatos, Gerasimos ;

Howard, Ian ;

Fischer, Armin ;

Hoogland, Sjoerd ;

Clifford, Jason ;

Klem, Ethan ;

Levina, Larissa ;

Sargent, Edward H. .

NATURE, 2006, 442 (7099) :180-183

[10]

Kowshik M, 2002, ADV MATER, V14, P815, DOI 10.1002/1521-4095(20020605)14:11<815::AID-ADMA815>3.0.CO