Relaxation rate distributions for supercooled liquids

被引:14
作者
Franosch, T [1 ]
Götze, W [1 ]
机构
[1] Tech Univ Munich, Dept Phys, D-85747 Garching, Germany
关键词
D O I
10.1021/jp983412r
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The mode-coupling theory for the evolution of glassy dynamics in simple liquids yields correlation functions that, outside the transient regime, can be written as a superposition of relaxators with a broad distribution of relaxation rates. The known asymptotic laws for the dynamics near an ideal glass transition imply corresponding laws for the rate distribution. We calculate the rate distributions for a hard-sphere liquid and compare them to the leading and next-to-leading asymptotic formulas.
引用
收藏
页码:4011 / 4017
页数:7
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