Will Solar-Driven Water-Splitting Devices See the Light of Day?

被引:625
作者
McKone, James R. [1 ,2 ]
Lewis, Nathan S. [1 ,2 ]
Gray, Harry B. [1 ,2 ]
机构
[1] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA
[2] CALTECH, Beckman Inst, Pasadena, CA 91125 USA
基金
美国国家科学基金会;
关键词
solar fuels; hydrogen evolution; HER; oxygen evolution; OER; photoelectrochemistry; electrocatalysis; semiconductor; ion-exchange membrane; SCANNING ELECTROCHEMICAL MICROSCOPY; OXYGEN-EVOLVING CATALYST; HYDROGEN-EVOLUTION; H-2; EVOLUTION; FUEL-CELLS; PHOTOASSISTED ELECTROLYSIS; PHOTO-CATHODES; PHOTOELECTROCHEMICAL CELLS; FUTURE CHALLENGES; ENERGY CONVERSION;
D O I
10.1021/cm4021518
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Through decades of sustained effort, researchers have made substantial progress on developing technologies for solar-driven water splitting. Nevertheless, more basic research is needed before prototype devices with a chance for commercial success can be demonstrated. In this Perspective, we summarize the major design constraints that motivate continued research in the field of solar-driven water splitting. Additionally, we discuss key device components that are now available for use in demonstration systems and prototypes. Finally, we highlight research areas where breakthroughs will be critical for continued progress toward commercial viability for solar-driven water-splitting devices.
引用
收藏
页码:407 / 414
页数:8
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