The importance of NOx production by lightning in the tropics

被引:112
作者
Bond, DW
Steiger, S
Zhang, RY [2 ]
Tie, XX
Orville, RE
机构
[1] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[2] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA
基金
美国国家科学基金会; 美国海洋和大气管理局; 美国国家航空航天局;
关键词
D O I
10.1016/S1352-2310(01)00553-2
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The importance of NOx production by lightning in the tropics has been assessed by using satellite lightning measurements from the Lightning Image Sensor (LIS). The lightning data from LIS over the period of 1998-2000 are analyzed and partitioned based on the latitude to obtain the numbers of cloud-to-ground (CG) and cloud-to-cloud (intracloud or IC) flashes. The average annual lightning counts over the 3-yr period are 3.0 x 10(8) CG flashes and 1.1 x 10(9) IC flashes between 35degreesN and 35degreesS. The resulting lightning distributions are employed to calculate the production of NOx. We obtain a lightning NOx production of 6.3TgNyr(-1) over this latitudinal region, using representative production values of 6.7 x 10(26) and 6.7 x 10(25) NO molecules for each CG and IC flash, respectively. NOx production by lightning varies slightly on a seasonal basis in accordance with the lightning distribution, with the maximum production occurring in the months of September, October, and November. The geographical and seasonal production of NOx by lightning is compared to NOx emissions from other sources (i.e., from anthropogenic activity, biomass burning, and soil emissions). The results indicate that production of NOx by tropical lightning is significant throughout the year. Lightning accounts for almost all of the NOx emitted over the oceans and 50-90% of NOx emitted over some continental areas on a seasonal basis. On the annual basis, the contribution of lightning to total NOx production is 23% in the tropics, and globally the lightning NOx production occurs predominately in this region. The uncertainty in estimating NOx production by lightning over the tropics is discussed. (C) 2002 Elsevier Science Ltd. All rights reserved.
引用
收藏
页码:1509 / 1519
页数:11
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