Cavity ring down spectroscopy with a free-electron laser

被引:22
作者
Engeln, R [1 ]
vandenBerg, E [1 ]
Meijer, G [1 ]
Lin, L [1 ]
Knippels, GMH [1 ]
vanderMeer, AFG [1 ]
机构
[1] EURATOM,FOM,INST PLASMAFYS RIJNHUIZEN,NL-3430 BE NIEUWEGEIN,NETHERLANDS
关键词
D O I
10.1016/S0009-2614(97)00292-3
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A cavity ring down (CRD) absorption experiment is performed with a free-electron laser (FEL) operating in the 10-11 mu m region. A short infrared pulse of approximately 20 ns, sliced from the much longer FEL pulse, is used to measure CRD spectra of ethylene in two different ways. First, ''ordinary'' CRD spectra with a resolution determined by the bandwidth of the FEL (approximate to 5 cm(-1)) are recorded, Second, Fourier transform (FT) CRD spectra with a resolution that is in principle determined by the FT-spectrometer are obtained by analyzing the light exiting the ring down cavity with a FT-spectrometer while the FEL is operated in broadband mode. (C) 1997 Elsevier Science B.V.
引用
收藏
页码:293 / 297
页数:5
相关论文
共 16 条
[1]   ULTRA-FAST SWITCHING OF INFRARED RADIATION BY LASER-PRODUCED CARRIERS IN SEMICONDUCTORS [J].
ALCOCK, AJ ;
CORKUM, PB .
CANADIAN JOURNAL OF PHYSICS, 1979, 57 (09) :1280-1290
[2]   KINETICS OF THE NH2+NO REACTION - EFFECTS OF TEMPERATURE ON THE TOTAL RATE-CONSTANT AND THE OH/H2O BRANCHING RATIO [J].
DIAU, EW ;
YU, T ;
WAGNER, MAG ;
LIN, MC .
JOURNAL OF PHYSICAL CHEMISTRY, 1994, 98 (15) :4034-4042
[3]   A Fourier transform cavity ring down spectrometer [J].
Engeln, R ;
Meijer, G .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1996, 67 (08) :2708-2713
[4]   TIME-RESOLVED FOURIER-TRANSFORM SPECTROSCOPY WITH 0.25 CM-1 SPECTRAL AND LESS-THAN-10(-7)S TIME RESOLUTION IN THE VISIBLE REGION [J].
HARTLAND, GV ;
XIE, W ;
DAI, HL ;
SIMON, A ;
ANDERSON, MJ .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1992, 63 (06) :3261-3267
[5]   BRANCH INTENSITIES AND OSCILLATOR-STRENGTHS FOR THE HERZBERG ABSORPTION SYSTEMS IN OXYGEN [J].
HUESTIS, DL ;
COPELAND, RA ;
KNUTSEN, K ;
SLANGER, TG ;
JONGMA, RT ;
BOOGAARTS, MGH ;
MEIJER, G .
CANADIAN JOURNAL OF PHYSICS, 1994, 72 (11-12) :1109-1121
[6]   2-COLOR FREE-ELECTRON LASER OPERATION [J].
JAROSZYNSKI, DA ;
PRAZERES, R ;
GLOTIN, F ;
ORTEGA, JM .
PHYSICAL REVIEW LETTERS, 1994, 72 (15) :2387-2390
[7]   TRACE GAS-DETECTION WITH CAVITY RING DOWN SPECTROSCOPY [J].
JONGMA, RT ;
BOOGAARTS, MGH ;
HOLLEMAN, I ;
MEIJER, G .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1995, 66 (04) :2821-2828
[8]   INTENSE FAR-INFRARED FREE-ELECTRON LASER-PULSES WITH A LENGTH OF 6 OPTICAL CYCLES [J].
KNIPPELS, GMH ;
MOLS, RFXAM ;
VANDERMEER, AFG ;
OEPTS, D ;
VANAMERSFOORT, PW .
PHYSICAL REVIEW LETTERS, 1995, 75 (09) :1755-1758
[9]   WAVELENGTH SHIFTING IN THE STANFORD FEL [J].
MARZIALI, A ;
SMITH, TI ;
SCHWETTMAN, HA .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1995, 358 (1-3) :252-255
[10]   COHERENT CAVITY RING DOWN SPECTROSCOPY [J].
MEIJER, G ;
BOOGAARTS, MGH ;
JONGMA, RT ;
PARKER, DH ;
WODTKE, AM .
CHEMICAL PHYSICS LETTERS, 1994, 217 (1-2) :112-116