Optical centrifuge for molecules

被引:243
作者
Karczmarek, J
Wright, J
Corkum, P
Ivanov, M
机构
[1] Natl Res Council Canada, Steacie Inst Mol Sci, Ottawa, ON K1A 0R6, Canada
[2] Carleton Univ, Ottawa Carleton Chem Inst, Ottawa, ON K1S 5B6, Canada
关键词
D O I
10.1103/PhysRevLett.82.3420
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Strong infrared fields can be used for controlled spinning of molecules to very high angular momentum states. The angular momentum acquired can be sufficient to break molecular bonds. The approach is suitable for all anisotropic molecules, and we illustrate it by dissociating a homonuclear diatomic Cl-2, with optical centrifuge efficiently separating Cl-35 and Cl-37 isotopes and thus demonstrating high sensitivity to the moment of inertia.
引用
收藏
页码:3420 / 3423
页数:4
相关论文
共 22 条
[1]  
[Anonymous], 1985, Journal of Molecular Structure: THEOCHEM
[2]   OBSERVATION OF A SINGLE-BEAM GRADIENT FORCE OPTICAL TRAP FOR DIELECTRIC PARTICLES [J].
ASHKIN, A ;
DZIEDZIC, JM ;
BJORKHOLM, JE ;
CHU, S .
OPTICS LETTERS, 1986, 11 (05) :288-290
[3]   Nonspreading wave packets for Rydberg electrons in rotating molecules with electric dipole moments [J].
BialynickiBirula, I ;
BialynickaBirula, Z .
PHYSICAL REVIEW LETTERS, 1996, 77 (21) :4298-4301
[4]   LAGRANGE EQUILIBRIUM POINTS IN CELESTIAL MECHANICS AND NONSPREADING WAVE-PACKETS FOR STRONGLY DRIVEN RYDBERG ELECTRONS [J].
BIALYNICKIBIRULA, I ;
KALINSKI, M ;
EBERLY, JH .
PHYSICAL REVIEW LETTERS, 1994, 73 (13) :1777-1780
[5]   Nonstationary, nondispersive wave packets in a Rydberg atom [J].
Brunello, AF ;
Uzer, T ;
Farrelly, D .
PHYSICAL REVIEW LETTERS, 1996, 76 (16) :2874-2877
[6]   EFFICIENT MOLECULAR DISSOCIATION BY A CHIRPED ULTRASHORT INFRARED-LASER PULSE [J].
CHELKOWSKI, S ;
BANDRAUK, AD ;
CORKUM, PB .
PHYSICAL REVIEW LETTERS, 1990, 65 (19) :2355-2358
[7]   CONTROL OF MOLECULAR VIBRATIONAL-EXCITATION AND DISSOCIATION BY CHIRPED INTENSE INFRARED-LASER PULSES - ROTATIONAL EFFECTS [J].
CHELKOWSKI, S ;
BANDRAUK, AD .
JOURNAL OF CHEMICAL PHYSICS, 1993, 99 (06) :4279-4287
[8]   ALIGNMENT AND TRAPPING OF MOLECULES IN INTENSE LASER FIELDS [J].
FRIEDRICH, B ;
HERSCHBACH, D .
PHYSICAL REVIEW LETTERS, 1995, 74 (23) :4623-4626
[9]   Optical alignment and spinning of laser-trapped microscopic particles [J].
Friese, MEJ ;
Nieminen, TA ;
Heckenberg, NR ;
Rubinsztein-Dunlop, H .
NATURE, 1998, 394 (6691) :348-350
[10]  
FRISCH MJ, 1994, GAUSSIAN 94 REV B 3