Anthropogenic emissions of methane in the United States

被引:399
作者
Miller, Scot M. [1 ]
Wofsy, Steven C. [1 ]
Michalak, Anna M. [2 ]
Kort, Eric A. [3 ]
Andrews, Arlyn E. [4 ]
Biraud, Sebastien C. [5 ]
Dlugokencky, Edward J. [4 ]
Eluszkiewicz, Janusz [7 ]
Fischer, Marc L. [6 ]
Janssens-Maenhout, Greet [8 ]
Miller, Ben R. [9 ]
Miller, John B. [9 ]
Montzka, Stephen A. [4 ]
Nehrkorn, Thomas [7 ]
Sweeney, Colm [9 ]
机构
[1] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA
[2] Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94305 USA
[3] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA
[4] NOAA, Global Monitoring Div, Earth Syst Res Lab, Boulder, CO 80305 USA
[5] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA
[6] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA
[7] Atmospher & Environm Res, Lexington, MA 02421 USA
[8] Commiss European Communities, Joint Res Ctr, Inst Environm & Sustainabil, I-21027 Ispra, Italy
[9] Univ Colorado Boulder, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
基金
美国国家科学基金会;
关键词
climate change policy; geostatistical inverse modeling; GEOSTATISTICAL APPROACH; ATMOSPHERIC METHANE; NITROUS-OXIDE; CO2; POLLUTION; DECADES;
D O I
10.1073/pnas.1314392110
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
This study quantitatively estimates the spatial distribution of anthropogenic methane sources in the United States by combining comprehensive atmospheric methane observations, extensive spatial datasets, and a high-resolution atmospheric transport model. Results show that current inventories from the US Environmental Protection Agency (EPA) and the Emissions Database for Global Atmospheric Research underestimate methane emissions nationally by a factor of similar to 1.5 and similar to 1.7, respectively. Our study indicates that emissions due to ruminants and manure are up to twice the magnitude of existing inventories. In addition, the discrepancy in methane source estimates is particularly pronounced in the south-central United States, where we find total emissions are similar to 2.7 times greater than in most inventories and account for 24 +/- 3% of national emissions. The spatial patterns of our emission fluxes and observed methane-propane correlations indicate that fossil fuel extraction and refining are major contributors (45 +/- 13%) in the south-central United States. This result suggests that regional methane emissions due to fossil fuel extraction and processing could be 4.9 +/- 2.6 times larger than in EDGAR, the most comprehensive global methane inventory. These results cast doubt on the US EPA's recent decision to downscale its estimate of national natural gas emissions by 25-30%. Overall, we conclude that methane emissions associated with both the animal husbandry and fossil fuel industries have larger greenhouse gas impacts than indicated by existing inventories.
引用
收藏
页码:20018 / 20022
页数:5
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