Measurement of anisotropy in the lateral momentum of a vibrating adsorbed molecule: CO/Cu(110)

被引:19
作者
Ahner, J [1 ]
Mocuta, D [1 ]
Ramsier, RD [1 ]
Yates, JT [1 ]
机构
[1] UNIV PITTSBURGH,DEPT PHYS,CTR SURFACE SCI,PITTSBURGH,PA 15260
关键词
D O I
10.1103/PhysRevLett.79.1889
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Anisotropies in the frustrated translational mode of CO chemisorbed on Cu(110) have been measured for the first time, with energies of 4.9 meV in the [1 (1) over bar 0] directions and 3.1 meV in the [001] directions. The measurements are made using a new time-of-flight ESDIAD (electron stimulated desorption ion angular distribution) method, permitting the resolution of bond directional effects and initial. state lateral momentum effects in ESDIAD patterns. These measurements provide a more detailed understanding of the librational potential energy well shape than has been possible previously.
引用
收藏
页码:1889 / 1892
页数:4
相关论文
共 21 条
[1]   Adsorbate-adsorbate repulsions - The coverage dependence of the adsorption structure of CO on Cu(110) as studied by electron-stimulated desorption ion angular distribution [J].
Ahner, J ;
Mocuta, D ;
Ramsier, RD ;
Yates, JT .
JOURNAL OF CHEMICAL PHYSICS, 1996, 105 (15) :6553-6559
[2]   THE DIRECT OBSERVATION OF HINDERED ROTATION OF A CHEMISORBED MOLECULE - PF3 ON NI(111) [J].
ALVEY, MD ;
YATES, JT ;
URAM, KJ .
JOURNAL OF CHEMICAL PHYSICS, 1987, 87 (12) :7221-7228
[3]   CONFORMATIONAL-CHANGES IN CHEMISORBED CO ON NI(110) DUE TO MOLECULAR-INTERACTIONS - AN ESDIAD STUDY [J].
ALVEY, MD ;
DRESSER, MJ ;
YATES, JT .
SURFACE SCIENCE, 1986, 165 (2-3) :447-465
[4]  
ALVEY MD, 1986, J VAC SCI TECHNOL A, V4, P1446
[5]   A He-atom scattering study of the frustrated translational mode of CO chemisorbed on defects on copper surfaces [J].
Braun, J ;
Graham, AP ;
Hofmann, F ;
Silvestri, W ;
Toennies, JP ;
Witte, G .
JOURNAL OF CHEMICAL PHYSICS, 1996, 105 (08) :3258-3263
[6]   DESORPTION BY ELECTRONICALLY STIMULATED ADSORBATE ROTATION [J].
BURNS, AR ;
STECHEL, EB ;
JENNISON, DR .
PHYSICAL REVIEW LETTERS, 1987, 58 (03) :250-253
[7]   QUANTUM SCATTERING THEORY OF ELECTRON-STIMULATED DESORPTION - ION ANGULAR-DISTRIBUTIONS [J].
CLINTON, WL .
PHYSICAL REVIEW LETTERS, 1977, 39 (15) :965-968
[8]   THE INTERACTION OF CO WITH COPPER (110) STUDIED BY TDS AND LEED [J].
HARENDT, C ;
GOSCHNICK, J ;
HIRSCHWALD, W .
SURFACE SCIENCE, 1985, 152 (APR) :453-462
[9]  
HOFMANN P, 1995, SURF SCI, V337, P169, DOI 10.1016/0039-6028(95)00612-5
[10]   X-RAY PHOTOELECTRON DIFFRACTION DETERMINATION OF THE MOLECULAR-ORIENTATION OF CO AND METHOXY ADSORBED ON CU(110) [J].
HOLUBKRAPPE, E ;
PRINCE, KC ;
HORN, K ;
WOODRUFF, DP .
SURFACE SCIENCE, 1986, 173 (01) :176-193