CO oxidation over a Pt/CoOx/SiO2 catalyst: A study using temporal analysis of products

被引:80
作者
Mergler, YJ [1 ]
Hoebink, J [1 ]
Nieuwenhuys, BE [1 ]
机构
[1] LEIDEN UNIV,LEIDEN INST CHEM,GORLAEUS LABS,NL-2300 RA LEIDEN,NETHERLANDS
关键词
D O I
10.1006/jcat.1997.1599
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Pt/CoOx/SiO2 catalysts consisting of 5 wt% Pt and 3 wt% Co3O4 are highly active for CO oxidation below 100 degrees C, In the present study the technique of temporal analysis of products was used to obtain information on the mechanism of the high activity, The behaviour of a 3 wt% CoOx/SiO2 and a 5 wt% Pt/SiO2 catalyst was compared with that of a Pt/CoOx/SiO2 catalyst. Several models proposed to explain the high activity of the Pt/CoOx/SiO2 catalyst are discussed. (C) 1997 Academic Press.
引用
收藏
页码:305 / 313
页数:9
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