Indian Ocean Experiment: An integrated analysis of the climate forcing and effects of the great Indo-Asian haze

被引:1108
作者
Ramanathan, V [1 ]
Crutzen, PJ
Lelieveld, J
Mitra, AP
Althausen, D
Anderson, J
Andreae, MO
Cantrell, W
Cass, GR
Chung, CE
Clarke, AD
Coakley, JA
Collins, WD
Conant, WC
Dulac, F
Heintzenberg, J
Heymsfield, AJ
Holben, B
Howell, S
Hudson, J
Jayaraman, A
Kiehl, JT
Krishnamurti, TN
Lubin, D
McFarquhar, G
Novakov, T
Ogren, JA
Podgorny, IA
Prather, K
Priestley, K
Prospero, JM
Quinn, PK
Rajeev, K
Rasch, P
Rupert, S
Sadourny, R
Satheesh, SK
Shaw, GE
Sheridan, P
Valero, FPJ
机构
[1] Univ Calif San Diego, Scripps Inst Oceanog, Ctr Atmospher Sci, La Jolla, CA 92037 USA
[2] Max Planck Inst Chem, D-55020 Mainz, Germany
[3] Natl Phys Lab, New Delhi 110012, India
[4] Inst Tropospher Res, D-04318 Leipzig, Germany
[5] Arizona State Univ, Dept Geol & Chem, Tempe, AZ 85287 USA
[6] Indiana Univ, Dept Chem, Bloomington, IN 47401 USA
[7] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA
[8] Univ Hawaii, Dept Oceanog, Honolulu, HI 96822 USA
[9] Oregon State Univ, Coll Ocean & Atmospher Sci, Corvallis, OR 97331 USA
[10] Natl Ctr Atmospher Res, Boulder, CO 80307 USA
[11] Lab Sci Climat & Environm, F-91191 Gif Sur Yvette, France
[12] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA
[13] Univ Nevada, Desert Res Inst, Reno, NV 89506 USA
[14] Phys Res Lab, Ahmadabad 380009, Gujarat, India
[15] Florida State Univ, Dept Meteorol, Tallahassee, FL 32306 USA
[16] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA
[17] NOAA, Climate Monitoring & Diagnost Lab, Boulder, CO 80303 USA
[18] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA
[19] NASA, Langley Res Ctr, Hampton, VA 23665 USA
[20] Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, Miami, FL 33149 USA
[21] NOAA, Pacific Marine Environm Lab, Seattle, WA 98115 USA
[22] Vikram Sarabhai Space Ctr, Space Phys Lab, Trivandrum 695022, Kerala, India
[23] Meteorol Dynam Lab, F-75005 Paris, France
[24] Univ Alaska Fairbanks, Inst Geophys, Fairbanks, AK 99775 USA
关键词
D O I
10.1029/2001JD900133
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Every year, from December to April, anthropogenic haze spreads over most of the North Indian Ocean, and South and Southeast Asia. The Indian Ocean Experiment (INDOEX) documented this Indo-Asian haze at scales ranging from individual particles to its contribution to the regional climate forcing. This study integrates the multiplatform. observations (satellites, aircraft, ships, surface stations, and balloons) with one- and four-dimensional models to derive the regional aerosol forcing resulting from the direct, the semidirect and the two indirect effects. The haze particles consisted of several inorganic and carbonaceous species, including absorbing black carbon clusters, fly ash, and mineral dust. The most striking result was the large loading of aerosols over most of the South Asian region and the North Indian Ocean. The January to March 1999 visible optical depths were about 0.5 over most of the continent and reached values as large as 0.2 over the equatorial Indian ocean due to long-range transport. The aerosol layer extended as high as 3 km. Black carbon contributed about 14% to the fine particle mass and 11% to the visible optical depth. The single-scattering albedo estimated by several independent methods was consistently around 0.9 both inland and over the open ocean. Anthropogenic sources contributed as much as 80% (+/- 10%) to the aerosol loading and the optical depth. The in situ data, which clearly support the existence of the first indirect effect (increased aerosol concentration producing more cloud drops with smaller effective radii), are used to develop a composite indirect effect scheme. The Indo-Asian aerosols impact the radiative forcing through a complex set of heating (positive forcing) and cooling (negative forcing) processes. Clouds and black carbon emerge as the ma or players. The dominant factor, however, is the large negative forcing (-20 +/- 4 W m(-2)) at the surface and the comparably large atmospheric heating. Regionally, the absorbing haze decreased the surface solar radiation by an amount comparable to 50% of the total ocean heat flux and nearly doubled the lower tropospheric solar heating. We demonstrate with a general circulation model how this additional heating significantly perturbs the tropical rainfall patterns and the hydrological cycle with implications to global climate.
引用
收藏
页码:28371 / 28398
页数:28
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