Teaching optimal control theory to distill robust pulses even under experimental constraints

被引：41

作者：

Hornung, T ^{[1
]}

Motzkus, M ^{[1
]}

de Vivie-Riedle, R ^{[1
]}

机构：

[1] MPI Quantenopt, D-85748 Garching, Germany

来源：

PHYSICAL REVIEW A | 2002年 / 65卷 / 02期

关键词：

D O I：

10.1103/PhysRevA.65.021403

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Optimal control theory (OCT) has wide applicability in the quest for seeking optimal laser pulses in coherent control of quantum phenomena. We have revised OCT making it possible to distill robust electric fields realizable via femtosecond pulse-shaping technology. The simple pulse structures offer direct physical insight into the control mechanism and selectively isolate the most stable pathways involving only few frequencies. Moreover, a generalized functional makes a vital extension in including the laser system used in control experiments.

引用

页数：4

共 16 条

[1] Molecular "π pulse" for total inversion of electronic state population
Cao, JS
Bardeen, CJ
Wilson, KR
[J]. PHYSICAL REVIEW LETTERS, 1998, 80 (07) : 1406 - 1409
[2] Selective preparation of enantiomers by laser pulses:: From optimal control to specific pump and dump transitions
González, L
Hoki, K
Kröner, D
Leal, AS
Manz, J
Ohtsuki, Y
[J]. JOURNAL OF CHEMICAL PHYSICS, 2000, 113 (24) : 11134 - 11142
[3] Driving wave packet recurrences with optimally modulated laser pulses
Goodson, BM
Goswami, D
Rabitz, H
Warren, WS
[J]. JOURNAL OF CHEMICAL PHYSICS, 2000, 112 (11) : 5081 - 5090
[4] Adapting optimal control theory and using learning loops to provide experimentally feasible shaping mask patterns
Hornung, T
Motzkus, M
de Vivie-Riedle, R
[J]. JOURNAL OF CHEMICAL PHYSICS, 2001, 115 (07) : 3105 - 3111
[5] Optimal control of molecular states in a learning loop with a parameterization in frequency and time domain
Hornung, T
Meier, R
Motzkus, M
[J]. CHEMICAL PHYSICS LETTERS, 2000, 326 (5-6) : 445 - 453
[6] TEACHING LASERS TO CONTROL MOLECULES
JUDSON, RS
RABITZ, H
[J]. PHYSICAL REVIEW LETTERS, 1992, 68 (10) : 1500 - 1503
[7] WAVEPACKET DANCING - ACHIEVING CHEMICAL SELECTIVITY BY SHAPING LIGHT-PULSES
KOSLOFF, R
RICE, SA
GASPARD, P
TERSIGNI, S
TANNOR, DJ
[J]. CHEMICAL PHYSICS, 1989, 139 (01) : 201 - 220
[8] Optimal control of molecular motion: Design, implementation, and inversion
Rabitz, H
Zhu, WS
[J]. ACCOUNTS OF CHEMICAL RESEARCH, 2000, 33 (08) : 572 - 578
[9] Chemistry - Whither the future of controlling quantum phenomena?
Rabitz, H
de Vivie-Riedle, R
Motzkus, M
Kompa, K
[J]. SCIENCE, 2000, 288 (5467) : 824 - 828
[10] Optical creation of vibrational intrinsic localized modes in anharmonic lattices with realistic interatomic potentials
Rössler, T
Page, JB
[J]. PHYSICAL REVIEW B, 2000, 62 (17): : 11460 - 11472

← 1 2 →