Scale-up analysis and development of gliding arc discharge facility for volatile organic compounds decomposition

被引:35
作者
Bo, Zheng [1 ]
Yan, Jianhua [1 ]
Li, Xiaodong [1 ]
Chi, Yong [1 ]
Cen, Kefa [1 ]
机构
[1] Zhejiang Univ, State Key Lab Clean Energy Utilizat, Inst Thermal Power Engn, Hangzhou 310003, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
gliding arc discharge; scale-up; decomposition; volatile organic compounds; non-thermal plasma;
D O I
10.1016/j.jhazmat.2007.11.105
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The influences of inlet gas flow rate and reactor configuration on volatile organic compounds (VOCs) decomposition efficiency in a traditional gliding arc (T-GA) facility are studied based on laboratory experiments and numerical simulation. The ratio of the nozzle diameter and the shortest distance of two electrodes should be maintained in a suitable value range to guarantee the decomposition efficiency, which indicates simply enlarging the nozzle inner diameter is not a proper way to raise the T-GA treatment capacity in a fixed supply voltage condition. A developed gliding arc gas discharge (D-GA) reactor based on a modified gas feed system is proposed: small flow rate air goes through the bottom nozzle to process the GA evolution, and high flow rate contaminated gas goes frontal through the plasma region and decomposes. The performances of D-GA reactor in the decomposition of VOCs with relative high gas flow rate, including decomposition efficiency and specific energy consumption, are better than T-GA reactor. D-GA reactor also avoids the drawbacks of the increases of power system amount and electric power consumption in multi-electrode GA system. (C) 2007 Elsevier B.V. All rights reserved.
引用
收藏
页码:494 / 501
页数:8
相关论文
共 21 条
[1]   Plasma treatment of aqueous solutes: Some chemical properties of a gliding arc in humid air [J].
Benstaali, B ;
Moussa, D ;
Addou, A ;
Brisset, JL .
EUROPEAN PHYSICAL JOURNAL-APPLIED PHYSICS, 1998, 4 (02) :171-179
[2]  
BO Z, 2006, ACTA SCI CIRCUMST, V26, P1
[3]   Effects of oxygen and water vapor on volatile organic compounds decomposition using gliding arc gas discharge [J].
Bo, Zh. ;
Yan, J. H. ;
Li, X. D. ;
Chi, Y. ;
Cen, K. F. ;
Cheron, B. G. .
PLASMA CHEMISTRY AND PLASMA PROCESSING, 2007, 27 (05) :546-558
[4]   GLIDING ARC - APPLICATIONS TO ENGINEERING AND ENVIRONMENT CONTROL [J].
CZERNICHOWSKI, A .
PURE AND APPLIED CHEMISTRY, 1994, 66 (06) :1301-1310
[5]  
CZERNICHOWSKI A, 1997, Patent No. 2763778
[6]  
CZERNICHOWSKI A, 1999, P 14 INT S PLASM CHE
[7]  
CZERNICHOWSKI A, 1996, CHEMTECH, V4, P45
[8]  
Delair L, 2001, HIGH TEMP MATER P-US, V5, P381
[9]   Gliding arc gas discharge [J].
Fridman, A ;
Nester, S ;
Kennedy, LA ;
Saveliev, A ;
Mutaf-Yardimci, O .
PROGRESS IN ENERGY AND COMBUSTION SCIENCE, 1999, 25 (02) :211-231
[10]  
GANGOLI S, 2005, ISPC 17