Lattice and magnetic instabilities in CaFe2As2:: A single-crystal neutron diffraction study

被引:286
作者
Goldman, A. I. [1 ,2 ]
Argyriou, D. N. [3 ]
Ouladdiaf, B.
Chatterji, T. [4 ]
Kreyssig, A. [1 ,2 ]
Nandi, S. [1 ,2 ]
Ni, N. [1 ,2 ]
Bud'ko, S. L. [1 ,2 ]
Canfield, P. C. [1 ,2 ]
McQueeney, R. J. [1 ,2 ]
机构
[1] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA
[2] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA
[3] Helmholtz Zentrum Berlin Mat & Energie, D-14109 Berlin, Germany
[4] Inst Max Von Laue Paul Langevin, Forschungszentrum, Julich Outstn, F-38042 Grenoble, France
来源
PHYSICAL REVIEW B | 2008年 / 78卷 / 10期
关键词
D O I
10.1103/PhysRevB.78.100506
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Neutron diffraction measurements of a high-quality single crystal of CaFe2As2 are reported. A sharp transition was observed between the high-temperature tetragonal and low-temperature orthorhombic structures at T-S=172.5 K (on cooling) and 173.5 K (on warming). Concomitant with the structural transition, the Fe moments order in a commensurate antiferromagnetic structure with a saturated moment of 0.80(5)mu(B)/Fe directed along the orthorhombic a axis. The hysteresis of both the structural and magnetic transitions is 1 K between cooling and warming, consistent with previous thermodynamic, transport, and single-crystal x-ray studies and provides clear evidence of the coupling between the structural and magnetic transitions in this material.
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相关论文
共 24 条
[1]  
Chen GF, 2008, CHINESE PHYS LETT, V25, P3403, DOI 10.1088/0256-307X/25/9/083
[2]   Superconductivity at 43 K in SmFeAsO1-xFx [J].
Chen, X. H. ;
Wu, T. ;
Wu, G. ;
Liu, R. H. ;
Chen, H. ;
Fang, D. F. .
NATURE, 2008, 453 (7196) :761-762
[3]   Magnetic order close to superconductivity in the iron-based layered LaO1-xFxFeAs systems [J].
de la Cruz, Clarina ;
Huang, Q. ;
Lynn, J. W. ;
Li, Jiying ;
Ratcliff, W., II ;
Zarestky, J. L. ;
Mook, H. A. ;
Chen, G. F. ;
Luo, J. L. ;
Wang, N. L. ;
Dai, Pengcheng .
NATURE, 2008, 453 (7197) :899-902
[4]  
HUANG Q, ARXIV08062776
[5]  
JESCHE A, ARXIV08070632
[6]   Iron-based layered superconductor La[O1-xFx]FeAs (x=0.05-0.12) with Tc=26 K [J].
Kamihara, Yoichi ;
Watanabe, Takumi ;
Hirano, Masahiro ;
Hosono, Hideo .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2008, 130 (11) :3296-+
[7]   Magnetic and structural transitions in layered iron arsenide systems:: AFe2As2 versus RFeAsO [J].
Krellner, C. ;
Caroca-Canales, N. ;
Jesche, A. ;
Rosner, H. ;
Ormeci, A. ;
Geibel, C. .
PHYSICAL REVIEW B, 2008, 78 (10)
[8]   Unconventional superconductivity with a sign reversal in the order parameter of LaFeAsO1-xFx [J].
Mazin, I. I. ;
Singh, D. J. ;
Johannes, M. D. ;
Du, M. H. .
PHYSICAL REVIEW LETTERS, 2008, 101 (05)
[9]   DOMAIN AND CRYSTAL-STRUCTURE OF SUPERCONDUCTING BA2YCU3O8-DELTA AT 40-K AND 100-K BY SINGLE-CRYSTAL NEUTRON-DIFFRACTION [J].
MCINTYRE, GJ ;
RENAULT, A ;
COLLIN, G .
PHYSICAL REVIEW B, 1988, 37 (10) :5148-5157
[10]   TWINNED CRYSTALS AND POSITION-SENSITIVE DETECTORS - A FITTING SOLUTION TO SINGLE-CRYSTAL STRUCTURAL STUDIES OF HIGH-TC SUPERCONDUCTORS [J].
MCINTYRE, GJ ;
RENAULT, A .
PHYSICA B, 1989, 156 :880-883