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PCDD/F and PCB multi-media ambient concentrations, congener patterns and occurrence in a Mediterranean coastal lagoon (Etang de Thau, France)
被引:61
作者:
Castro-Jimenez, J.
[1
]
Deviller, G.
[1
]
Ghiani, A.
[1
]
Loos, R.
[1
]
Mariani, G.
[1
]
Skejo, H.
[1
]
Umlauf, G.
[1
]
Wollgast, J.
[1
]
Laugier, T.
[2
]
Heas-Moisan, K.
[3
]
Leaute, F.
[3
]
Munschy, C.
[3
]
Tixier, C.
[3
]
Tronczynski, J.
[3
]
机构:
[1] European Commiss DG, Joint Res Ctr, IES, I-21020 Ispra, VA, Italy
[2] IFREMER, Lab Environm Resources, F-34203 Sete, France
[3] IFREMER, Lab Biogeochem Organ Contaminants, F-44311 Nantes 3, France
关键词:
POPs;
Air Sediment;
Mussel;
Water column;
D O I:
10.1016/j.envpol.2007.12.019
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Ambient concentrations, congener patterns and multi-media distribution of PCDD/Fs and PCBs were determined in air, water, sediment and mussels in a semi-enclosed marine ecosystem (Thau lagoon, France). Sigma 2,3,7,8-PCDD/F and Sigma 7ICES PCB air concentrations (0.2-1.4 and 31-57 pg m(-3), respectively) were typical of rural areas. Concentrations in the water column were very low for PCDD/Fs (163-476 fg L-1) and low for PCBs (138-708 pg L-1). PCDD/F and PCB concentrations found in surface sediment (0.15-1.6 and 2.5-33 ng g(-1) d.w., respectively) and mussel (13-21 pg g(-1) d.w. and 10-39 ng g(-1) d.w., respectively) were medium levels. PCDD/F congener patterns observed in air, water particulate phase and sediments were similar suggesting direct coupling among these compartments and atmospheric inputs of PCDD/Fs into the lagoon. Conversely, for the same set of samples, similar patterns were not observed for PCBs in the mentioned compartments. (C) 2007 Elsevier Ltd. All rights reserved.
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页码:123 / 135
页数:13
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