Characteristics of Elemental Composition of PM2.5 in the Spring Period at Tongyu in the Semi-arid Region of Northeast China

被引:34
作者
Zhang Renjian [1 ]
Fu Congbin [1 ]
Han Zhiwei [1 ]
Zhu Chongshu [2 ]
机构
[1] Chinese Acad Sci, START Reg Ctr Temperate E Asia, Inst Atmospher Phys, Key Lab Reg Climate Environm Res Temperate E Asia, Beijing 100029, Peoples R China
[2] Chinese Acad Sci, Inst Earth Environm, SKLLQG, Xian 710075, Peoples R China
关键词
dust aerosol; mass concentration; elemental composition; transport pathway;
D O I
10.1007/s00376-008-0922-7
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Continuous observations of mass concentration and elemental composition of aerosol particles (PM2.5) were conducted at Tongyu, a semi-arid site in Northeast China in the spring of 2006. The average mass concentration of PM2.5 at Tongyu station was 260.9 +/- 274.4 mu g m(-3) during the observation period. Nine dust events were monitored with a mean concentration of 528.0 +/- 302.7 mu g m(-3). The PM2.5 level during non-dust storm (NDS) period was 111.65 +/- 63.37 mu g m(-3). High mass concentration shows that fine-size particles pollution was very serious in the semi-arid area in Northeast China. The enrichment factor values for crust elements during the dust storm (DS) period are close to those in the NDS period, while the enrichment factor values for pollution elements during the NDS period are much higher than those in the DS period, showing these elements were from anthropogenic sources. The ratios of dust elements to Fe were relative constant during the DS period. The Ca/Fe ratio in dust aerosols at, Tongyu is remarkably different from that observed in other source regions and downwind regions. Meteorological analysis shows that dust events at Tongyu are usually associated with dry, low pressure and high wind speed weather conditions. Air mass back-trajectory analysis identified three kinds of general pathways were associated with the aerosol particle transport to Tongyu, and the northwest direction pathway was the main transport route.
引用
收藏
页码:922 / 931
页数:10
相关论文
共 51 条
[1]   Chemical and optical characterization of aerosols measured in spring 2002 at the ACE-Asia supersite, Zhenbeitai, China [J].
Alfaro, SC ;
Gomes, L ;
Rajot, JL ;
Lafon, S ;
Gaudichet, A ;
Chatenet, B ;
Maille, M ;
Cautenet, G ;
Lasserre, F ;
Cachier, H ;
Zhang, XY .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
[2]   Strong present-day aerosol cooling implies a hot future [J].
Andreae, MO ;
Jones, CD ;
Cox, PM .
NATURE, 2005, 435 (7046) :1187-1190
[3]  
[Anonymous], 2019, THE J, DOI DOI 10.1590/0103-6440201902280
[4]  
[Anonymous], 2004, CHINA PARTICUOLOGY
[5]   Chemical composition of atmospheric aerosols from Zhenbeitai, China, and Gosan, South Korea, during ACE-Asia [J].
Arimoto, R ;
Zhang, XY ;
Huebert, BJ ;
Kang, CH ;
Savoie, DL ;
Prospero, JM ;
Sage, SK ;
Schloesslin, CA ;
Khaing, HM ;
Oh, SN .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D19) :D19S041-15
[6]   Characterization of airborne carbonate over a site near Asian dust source regions during spring 2002 and its climatic and environmental significance [J].
Cao, JJ ;
Lee, SC ;
Zhang, XY ;
Chow, JC ;
An, ZS ;
Ho, KF ;
Watson, JG ;
Fung, K ;
Wang, YQ ;
Shen, ZX .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2005, 110 (D3) :1-8
[7]   Chemical characteristics of Asian dust aerosol from Hunshan Dake sandland in Northern China [J].
Cheng, TT ;
Lu, DR ;
Wang, GC ;
Xu, YF .
ATMOSPHERIC ENVIRONMENT, 2005, 39 (16) :2903-2911
[8]   On heavy dustfall observed with explosive sandstorms in Chongwon-Chongju, Korea in 2002 [J].
Chung, YS ;
Kim, HS ;
Dulam, J ;
Harris, J .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (24) :3425-3433
[9]   Potential impacts of human-induced land cover change on East Asia monsoon [J].
Fu, CB .
GLOBAL AND PLANETARY CHANGE, 2003, 37 (3-4) :219-229
[10]   The elemental and organic characteristics of PM2.5 in Asian dust episodes in Qingdao, China, 2002 [J].
Guo, ZG ;
Feng, JL ;
Fang, M ;
Chen, HY ;
Lau, KH .
ATMOSPHERIC ENVIRONMENT, 2004, 38 (06) :909-919