Powering the future of molecular artificial photosynthesis with light-harvesting metallosupramolecular dye assemblies

被引：525

作者：

Frischmann, Peter D.

Mahata, Kingsuk

Wuerthner, Frank ^{[1
,2
]}

机构：

[1] Univ Wurzburg, Inst Organ Chem, D-97074 Wurzburg, Germany

[2] Ctr Nanosyst Chem, D-97074 Wurzburg, Germany

来源：

CHEMICAL SOCIETY REVIEWS | 2013年 / 42卷 / 04期

关键词：

PHOTOCATALYTIC HYDROGEN-PRODUCTION; RUTHENIUM PHTHALOCYANINE COMPLEXES; PHOTOINITIATED ELECTRON COLLECTION; RESONANCE ENERGY-TRANSFER; WATER OXIDATION CATALYST; PERYLENE BISIMIDE DYES; PHOTOSYSTEM-II; CRYSTAL-STRUCTURE; BUILDING-BLOCKS; MULTIPORPHYRIN ARRAYS;

D O I：

10.1039/c2cs35223k

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Chemical ingenuity will play a significant role in solving the greatest challenge currently facing society: providing clean and carbon neutral energy for all of humanity. Molecular artificial photosynthesis is an emerging technology based on principles learned from Nature where individual components perform the essential light-harvesting, charge-separation, and water splitting functions to store solar energy in the form of chemical bonds. This tutorial review focuses specifically on the application of metallosupramolecular self-assembly strategies to interface solar fuel catalysts with photosensitizers and construct light-harvesting antennae capable of achieving panchromatic absorption and directional energy concentration.

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页码：1847 / 1870

页数：24

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