Slowed relaxational dynamics beyond the fluctuation-dissipation theorem

被引:9
作者
De Gregorio, P [1 ]
Sciortino, F
Tartaglia, P
Zaccarelli, E
Dawson, KA
机构
[1] Univ Coll Dublin, Dept Chem, Irish Ctr Colloid Sci & Biomat, Dublin 4, Ireland
[2] INFM, Ctr Stat Mech & Complex, I-00185 Rome, Italy
[3] Univ Roma La Sapienza, Dipartimento Fis, INFM, I-00185 Rome, Italy
关键词
fluctuation-dissipation theorem; glasses; mode coupling theory; aging;
D O I
10.1016/S0378-4371(01)00398-3
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
To describe the slow dynamics of a system out of equilibrium, but close to a dynamical arrest, we generalise the ideas of previous work to the case where time-translational invariance is broken. We introduce a model of dynamics that is reasonably general, and show how all of the unknown parameters of this model may be related to the observables or to averages of the noise. One result is a generalisation of the Fluctuation-dissipation theorem of type two (FDT2), and the method is thereby freed from this constraint. Significantly, a systematic means of implementing the theory to higher order is outlined. We propose the simplest possible closure of these generalised equations, following the same type of approximations that have been long known for the equilibrium case of mode coupling theory (MCT). Naturally, equilibrium MCT equations are found as a limit of this generalised formalism. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:15 / 26
页数:12
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