Complete analysis of the Na3+ fragmentation in collision with He atoms

被引:18
作者
Barat, M
Brenot, JC
Dunet, H
Fayeton, JA
Picard, YJ
Babikov, D
Sizun, M
机构
[1] Univ Paris Sud XI, Collis Atom & Mol Lab, UMR C8625, F-91405 Orsay, France
[2] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia
基金
美国国家航空航天局; 美国国家科学基金会;
关键词
D O I
10.1016/S0009-2614(99)00448-0
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
An experimental investigation of the fragmentation mechanisms of Na-3(+) cluster ions in collision with He atoms at 263 eV centre-of-mass energy is presented. The relative populations of the three fragmentation pathways are determined. In particular, the kinematics of the three-body breakup is studied in detail. The analysis of the correlation between the velocity vectors of the fragments allows one to estimate the relative role of the electronic excitation or momentum transfer in the population of each pathway. The discussion of the fragmentation dynamics is based on a concomitant theoretical study. (C) 1999 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:233 / 238
页数:6
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