Photoionization of metal clusters

被引:20
作者
Koskinen, M [1 ]
Manninen, M [1 ]
机构
[1] UNIV JYVASKYLA,DEPT PHYS,FIN-40351 JYVASKYLA,FINLAND
来源
PHYSICAL REVIEW B | 1996年 / 54卷 / 20期
关键词
D O I
10.1103/PhysRevB.54.14796
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The photoionization cross section of metal clusters is studied using simple theoretical models. In the case of small clusters, the plasmon is well below the photoionization threshold and the photoionization is dominated by simple independent-particle processes: One electron absorbs all the energy of the photon and immediately leaves the cluster. For large sodium clusters the photoionization efficiency curve is a result of a two-step process: First, the photon excites a plasmon and then the plasmon decays, either by emitting a photoelectron or by heating the cluster. A simple expression for the photoionization cross section near the threshold is derived.
引用
收藏
页码:14796 / 14806
页数:11
相关论文
共 19 条
[1]   OBSERVATION OF ELECTRONIC SHELL STRUCTURE IN LARGE CESIUM OXIDE CLUSTERS [J].
BERGMANN, T ;
MARTIN, TP .
JOURNAL OF CHEMICAL PHYSICS, 1989, 90 (06) :2848-2855
[2]   SIMPLE METAL-CLUSTERS [J].
BRECHIGNAC, C ;
CAHUZAC, P ;
CARLIER, F ;
DEFRUTOS, M ;
LEYGNIER, J .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1991, 19 (1-4) :1-6
[3]   IONIZATION VS NEUTRALIZATION IN ALKALI-ATOM CLUSTERS [J].
BRECHIGNAC, C ;
CAHUZAC, P ;
CARLIER, F ;
DEFRUTOS, M ;
LEYGNIER, J ;
ROUX, JP ;
SARFATI, A .
JOURNAL DE PHYSIQUE II, 1992, 2 (04) :971-983
[4]  
EATON JG, 1992, NATO ADV STUDY I C, V1, P493
[5]   The analysis of photoelectric sensitivity curves for clean metals at various temperatures [J].
Fowler, RH .
PHYSICAL REVIEW, 1931, 38 (01) :45-56
[6]   IONIZATION ENERGIES OF SODIUM CLUSTERS CONTAINING UP TO 22000 ATOMS [J].
GOHLICH, H ;
LANGE, T ;
BERGMANN, T ;
NAHER, U ;
MARTIN, TP .
CHEMICAL PHYSICS LETTERS, 1991, 187 (1-2) :67-72
[7]   SODIUM CLUSTER IONIZATION-POTENTIALS REVISITED - HIGHER-RESOLUTION MEASUREMENTS FOR NAX (X-LESS-THAN-23) AND THEIR RELATION TO BONDING MODELS [J].
KAPPES, MM ;
SCHAR, M ;
ROTHLISBERGER, U ;
YERETZIAN, C ;
SCHUMACHER, E .
CHEMICAL PHYSICS LETTERS, 1988, 143 (03) :251-258
[8]   MANY-BODY ORIGIN OF THE PLASMON RESONANCE IN SMALL METAL-CLUSTERS [J].
KOSKINEN, M ;
MANNINEN, M ;
LIPAS, PO .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1994, 31 (1-2) :125-129
[9]   PHOTOIONIZATION OF SODIUM CLUSTERS [J].
PETERSON, KI ;
DAO, PD ;
FARLEY, RW ;
CASTLEMAN, AW .
JOURNAL OF CHEMICAL PHYSICS, 1984, 80 (05) :1780-1785
[10]  
REINERS T, UNPUB