H-2 oxidation at the interface Ni/Sr0.995Ce0.95Y0.05O2.975

被引:24
作者
Bonanos, N
Mogensen, M
机构
关键词
perovskite; anode; polarisation; limiting current;
D O I
10.1016/S0167-2738(97)00052-0
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The oxidation of hydrogen at the interface of nickel and the perovskite proton conductor Sr0.995Ce0.95Y0.05O2.975 has been investigated at 800 degrees C and below in atmospheres of N-2/H-2/H2O, using a point contact electrode technique. The polarisation behaviour obtained in the anodic regime suggested the transport of a species undergoing one electron transfer. Limiting currents were dependent on the partial pressure of hydrogen, but not on that of water vapour.
引用
收藏
页码:483 / 488
页数:6
相关论文
共 16 条
[1]  
AHLGREN EO, 1996, P 17 RIS INT S MAT S, P161
[2]   OXIDE ION CONDUCTION IN YTTERBIUM-DOPED STRONTIUM CERATE [J].
BONANOS, N ;
ELLIS, B ;
MAHMOOD, MN .
SOLID STATE IONICS, 1988, 28 :579-584
[3]   ELECTROCATALYTIC NONOXIDATIVE DIMERIZATION OF METHANE OVER AG ELECTRODES [J].
CHIANG, PH ;
ENG, D ;
STOUKIDES, M .
SOLID STATE IONICS, 1993, 61 (1-3) :99-103
[4]  
GUINDET J, 1991, THESIS I NATL POLYTE
[5]  
IWAHARA H, 1992, SOLID STATE IONICS //, P575
[7]   ELECTRICAL-PROPERTIES OF SRCE0.95YB0.05O3 IN HYDROGEN CONTAINING ATMOSPHERES [J].
KOSACKI, I ;
BECHT, JGM ;
VANLANDSCHOOT, R ;
SCHOONMAN, J .
SOLID STATE IONICS, 1993, 59 (3-4) :287-296
[8]   IN-SITU MEASUREMENTS OF THE WATER-UPTAKE IN YB DOPED SRCEO3 [J].
KRUG, F ;
SCHOBER, T ;
SPRINGER, T .
SOLID STATE IONICS, 1995, 81 (1-2) :111-118
[9]  
MAHMOOD MN, 1992, SOLID STATE IONICS, V53, P141
[10]   RESISTANCE FOR FLOW OF CURRENT TO A DISK [J].
NEWMAN, J .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 1966, 113 (05) :501-&