Bulk- and surface-sensitive high-resolution photoemission study of two mott-hubbard systems: SrVO3 and CaVO3

被引:64
作者
Eguchi, R [1 ]
Kiss, T
Tsuda, S
Shimojima, T
Mizokami, T
Yokoya, T
Chainani, A
Shin, S
Inoue, IH
Togashi, T
Watanabe, S
Zhang, CQ
Chen, CT
Arita, M
Shimada, K
Namatame, H
Taniguchi, M
机构
[1] Univ Tokyo, ISSP, Kashiwa, Chiba 2778581, Japan
[2] RIKEN, SPring Ctr 8, Sayo, Hyogo 6795148, Japan
[3] AIST, CERC, Tsukuba, Ibaraki 3058562, Japan
[4] Chinese Acad Sci, Beijing Ctr Crystal R&D, Beijing 100080, Peoples R China
[5] Hiroshima Univ, Ctr Synchrotron Radiat, Higashihiroshima 7398526, Japan
[6] Hiroshima Univ, Grad Sch Sci, Higashihiroshima 7398526, Japan
关键词
D O I
10.1103/PhysRevLett.96.076402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We study the electronic structure of Mott-Hubbard systems SrVO3 and CaVO3 with bulk and surface-sensitive high-resolution photoemission spectroscopy, using a vacuum ultraviolet laser, synchrotron radiation, and a discharge lamp (h nu=7-21 eV). A systematic suppression of the density of states (DOS) within similar to 0.2 eV of the Fermi level (E-F) is found on decreasing photon energy, i.e., on increasing bulk sensitivity. The coherent band in SrVO3 and CaVO3 is shown to consist of surface and bulk-derived features, separated in energy. The stronger distortion on surface of CaVO3 compared to SrVO3 leads to a higher surface metallicity in the coherent DOS at E-F, consistent with recent theory.
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页数:4
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