Theory of time-resolved photoelectron imaging: Nonperturbative calculation for an internally converting polyatomic molecule

被引:21
作者
Suzuki, Y
Stener, M
Seideman, T
机构
[1] Natl Res Council Canada, Steacie Inst Mol Sci, Ottawa, ON K1A 0R6, Canada
[2] Univ Trieste, Dipartimento Sci Chim, I-34127 Trieste, Italy
关键词
D O I
10.1103/PhysRevLett.89.233002
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present the first calculation of time-resolved photoelectron angular distributions for a polyatomic system. Our method takes rotations into exact account, treats the laser field nonperturbatively, and computes the electronic dynamics from first principles. Our results point to the information content of time-resolved photoelectron imaging observables and illustrate the role played by the field intensity.
引用
收藏
页码:1 / 233002
页数:4
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