Spin waves and quantum criticality in the frustrated XY pyrochlore antiferromagnet Er2Ti2O7

被引:83
作者
Ruff, J. P. C. [1 ]
Clancy, J. P. [1 ]
Bourque, A. [2 ]
White, M. A. [2 ]
Ramazanoglu, M. [1 ]
Gardner, J. S. [3 ,4 ]
Qiu, Y. [3 ,5 ]
Copley, J. R. D. [3 ]
Johnson, M. B. [2 ]
Dabkowska, H. A. [1 ]
Gaulin, B. D. [1 ,6 ]
机构
[1] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada
[2] Dalhousie Univ, Dept Chem, Inst Mat Res, Halifax, NS B3H 4J3, Canada
[3] Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA
[4] Indiana Univ, Bloomington, IN 47408 USA
[5] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA
[6] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada
基金
美国国家科学基金会; 加拿大自然科学与工程研究理事会;
关键词
D O I
10.1103/PhysRevLett.101.147205
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report detailed measurements of the low temperature magnetic phase diagram of Er2Ti2O7. Heat capacity and time- of- flight neutron scattering studies of single crystals reveal unconventional low- energy states. Er3+ magnetic ions reside on a pyrochlore lattice in Er2Ti2O7, where local XY anisotropy and antiferromagnetic interactions give rise to a unique frustrated system. In zero field, the ground state exhibits coexisting short and long- range order, accompanied by soft collective spin excitations previously believed to be absent. The application of finite magnetic fields tunes the ground state continuously through a landscape of noncollinear phases, divided by a zero temperature phase transition at mu(0)Hc similar to 1.5 T. The characteristic energy scale for spin fluctuations is seen to vanish at the critical point, as expected for a second order quantum phase transition driven by quantum fluctuations.
引用
收藏
页数:4
相关论文
共 18 条
[1]  
[Anonymous], 2000, QUANTUM PHASE TRANSI, DOI [DOI 10.1017/CBO9780511622540, DOI 10.1017/CBO9780511973765]
[2]   Quantum critical behavior for a model magnet [J].
Bitko, D ;
Rosenbaum, TF ;
Aeppli, G .
PHYSICAL REVIEW LETTERS, 1996, 77 (05) :940-943
[3]   HEAT-CAPACITY MEASUREMENTS ON RARE-EARTH DOUBLE OXIDES R2M2O7 [J].
BLOTE, HWJ ;
WIELINGA, RF ;
HUISKAMP, WJ .
PHYSICA, 1969, 43 (04) :549-&
[4]   Spin ice state in frustrated magnetic pyrochlore materials [J].
Bramwell, ST ;
Gingras, MJP .
SCIENCE, 2001, 294 (5546) :1495-1501
[5]   ORDER BY DISORDER IN AN ANISOTROPIC PYROCHLORE LATTICE ANTIFERROMAGNET [J].
BRAMWELL, ST ;
GINGRAS, MJP ;
REIMERS, JN .
JOURNAL OF APPLIED PHYSICS, 1994, 75 (10) :5523-5525
[6]   Magnetic monopoles in spin ice [J].
Castelnovo, C. ;
Moessner, R. ;
Sondhi, S. L. .
NATURE, 2008, 451 (7174) :42-45
[7]   Er2Ti2O7:: Evidence of quantum order by disorder in a frustrated antiferromagnet -: art. no. 020401 [J].
Champion, JDM ;
Harris, MJ ;
Holdsworth, PCW ;
Wills, AS ;
Balakrishnan, G ;
Bramwell, ST ;
Cizmár, E ;
Fennell, T ;
Gardner, JS ;
Lago, J ;
McMorrow, DF ;
Orendác, M ;
Orendácová, A ;
Paul, DM ;
Smith, RI ;
Telling, MTF ;
Wildes, A .
PHYSICAL REVIEW B, 2003, 68 (02)
[8]   The Disk Chopper Spectrometer at NIST: a new instrument for quasielastic neutron scattering studies [J].
Copley, JRD ;
Cook, JC .
CHEMICAL PHYSICS, 2003, 292 (2-3) :477-485
[9]  
Diep HT, 2005, FRUSTRATED SPIN SYSTEMS, P1, DOI 10.1142/9789812567819
[10]   Cooperative paramagnetism in the geometrically frustrated pyrochlore antiferromagnet Tb2Ti2O7 [J].
Gardner, JS ;
Dunsiger, SR ;
Gaulin, BD ;
Gingras, MJP ;
Greedan, JE ;
Kiefl, RF ;
Lumsden, MD ;
MacFarlane, WA ;
Raju, NP ;
Sonier, JE ;
Swainson, I ;
Tun, Z .
PHYSICAL REVIEW LETTERS, 1999, 82 (05) :1012-1015