A photoelectron diffraction study of the Pd{111}(root 3x root 3)R30 degrees-CO chemisorption phase

被引:19
作者
Fernandez, V
Giessel, T
Schaff, O
Schindler, KM
Theobald, A
Hirschmugl, CJ
Bao, S
Bradshaw, AM
Baddeley, C
Lee, AF
Lambert, RM
Woodruff, DP
Fritzsche, V
机构
[1] UNIV CAMBRIDGE,DEPT CHEM,CAMBRIDGE CB2 1EW,ENGLAND
[2] UNIV WARWICK,DEPT PHYS,COVENTRY CV4 7AL,W MIDLANDS,ENGLAND
[3] TECH UNIV DRESDEN,INST THEORET PHYS,D-01062 DRESDEN,GERMANY
来源
ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS | 1997年 / 198卷
关键词
adsorption; electron scattering; photoelectron spectroscopy; single crystals; surface structure;
D O I
10.1524/zpch.1997.198.Part_1_2.073
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Using scanned-energy mode photoelectron diffraction we show that in the Pd{111} (root 3 x root 3)R30 degrees-CO phase fee hollow sites are occupied with a carbon-Pd layer spacing of 1.27 (+/-0.05) Angstrom. This agrees very well with a relatively early LEED result of the Somorjai group and indicates that the experimental problems associated with applying scanned-energy mode photoelectron diffraction to second row transition metal substrates are not insurmountable.
引用
收藏
页码:73 / 85
页数:13
相关论文
共 26 条
[1]  
BERNDT WO, IN PRESS
[2]  
Bradshaw A. M., 1995, Applications of synchrotron radiation. High-resolution studies of molecules and molecular adsorbates on surfaces, P127
[3]   CHEMISORPTION OF CARBON-MONOXIDE ON PALLADIUM SINGLE-CRYSTAL SURFACES - IR SPECTROSCOPIC EVIDENCE FOR LOCALIZED SITE ADSORPTION [J].
BRADSHAW, AM ;
HOFFMANN, FM .
SURFACE SCIENCE, 1978, 72 (03) :513-535
[4]  
BUISSET J, IN PRESS PHYS REV B
[5]   INTERACTIONS BETWEEN OXYGEN AND CARBON-MONOXIDE ON A PD(111) SURFACE [J].
CONRAD, H ;
ERTL, G ;
KUPPERS, J .
SURFACE SCIENCE, 1978, 76 (02) :323-342
[6]   STRUCTURE DETERMINATION OF AN ALKALI-METAL CO COADSORPTION PHASE - NI(111)-K/CO [J].
DAVIS, R ;
WOODRUFF, DP ;
SCHAFF, O ;
FERNANDEZ, V ;
SCHINDLER, KM ;
HOFMANN, P ;
WEISS, KU ;
DIPPEL, R ;
FRITZSCHE, V ;
BRADSHAW, AM .
PHYSICAL REVIEW LETTERS, 1995, 74 (09) :1621-1624
[7]   A HIGH-FLUX TOROIDAL GRATING MONOCHROMATOR FOR THE SOFT-X-RAY REGION [J].
DIETZ, E ;
BRAUN, W ;
BRADSHAW, AM ;
JOHNSON, RL .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1985, 239 (02) :359-366
[8]  
DVIS R, 1996, J PHYS CONDENS MATT, V8, P1367
[9]   ADSORPTION OF CO ON A PALLADIUM(III) SURFACE [J].
ERTL, G ;
KOCH, J .
ZEITSCHRIFT FUR NATURFORSCHUNG PART A-ASTROPHYSIK PHYSIK UND PHYSIKALISCHE CHEMIE, 1970, A 25 (12) :1906-&
[10]   Structure determination of a CO/O coadsorption phase on Ni(111) [J].
Fernandez, V ;
Schindler, KM ;
Schaff, O ;
Hofmann, P ;
Theobald, A ;
Bradshaw, AM ;
Fritzsche, V ;
Davis, R ;
Woodruff, DP .
SURFACE SCIENCE, 1996, 351 (1-3) :1-12