Field-Induced Spin-Ice-Like Orders in Spin Liquid Tb2Ti2O7

被引:30
作者
Cao, H. [1 ]
Gukasov, A. [1 ]
Mirebeau, I. [1 ]
Bonville, P. [2 ]
Dhalenne, G. [3 ]
机构
[1] CE Saclay, CNRS, CEA, Leon Brillouin Lab, F-91191 Gif Sur Yvette, France
[2] CE Saclay, CNRS, CEA, Serv Phys Etat Condense, F-91191 Gif Sur Yvette, France
[3] Univ Paris 11, Lab Physicochim Etat Solide, F-91405 Orsay, France
关键词
D O I
10.1103/PhysRevLett.101.196402
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We have studied the field-induced magnetic structures in Tb(2)Ti(2)O(7), in a wide temperature (0.3 < T < 270 K) and field (0 < H < 7 T) range, by single crystal polarized and unpolarized neutron diffraction, with H parallel to[110] axis. A ferromagneticlike structure with k=0 propagation vector is induced, whose local order at low field and low temperature is akin to spin ice. The four Tb ions separate in alpha and beta chains having different values of the magnetic moments, which is quantitatively explained by taking the crystal field anisotropy into account. Above 2 T and below 2 K, an antiferromagneticlike structure with k=(0,0,1) is induced besides the k=0 structure. It shows a reentrant behavior and extends over a finite length scale. It occurs together with a broadening of the nuclear peaks, which suggests a field-induced distortion and magnetostriction effect.
引用
收藏
页数:4
相关论文
共 27 条
[1]  
Aleksandrov I. V., 1985, Soviet Physics - JETP, V62, P1287
[2]   Crystal structure under pressure of geometrically frustrated pyrochlores [J].
Apetrei, A. ;
Mirebeau, I. ;
Goncharenko, I. ;
Crichton, W. A. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2007, 19 (37)
[3]   Spin ice state in frustrated magnetic pyrochlore materials [J].
Bramwell, ST ;
Gingras, MJP .
SCIENCE, 2001, 294 (5546) :1495-1501
[4]  
BROWN PJ, 1993, CCSLRAL93009, P52409
[5]   Magnetic monopoles in spin ice [J].
Castelnovo, C. ;
Moessner, R. ;
Sondhi, S. L. .
NATURE, 2008, 451 (7174) :42-45
[6]   Theory of paramagnetic scattering in highly frustrated magnets with long-range dipole-dipole interactions:: The case of the Tb2Ti2O7 pyrochlore antiferromagnet -: art. no. 174426 [J].
Enjalran, M ;
Gingras, MJP .
PHYSICAL REVIEW B, 2004, 70 (17) :1-17
[7]   Neutron scattering studies of the spin ices Ho2Ti2O7 and Dy2Ti2O7 in applied magnetic field -: art. no. 224411 [J].
Fennell, T ;
Petrenko, OA ;
Fåk, B ;
Gardner, JS ;
Bramwell, ST ;
Ouladdiaf, B .
PHYSICAL REVIEW B, 2005, 72 (22)
[8]   Cooperative paramagnetism in the geometrically frustrated pyrochlore antiferromagnet Tb2Ti2O7 [J].
Gardner, JS ;
Dunsiger, SR ;
Gaulin, BD ;
Gingras, MJP ;
Greedan, JE ;
Kiefl, RF ;
Lumsden, MD ;
MacFarlane, WA ;
Raju, NP ;
Sonier, JE ;
Swainson, I ;
Tun, Z .
PHYSICAL REVIEW LETTERS, 1999, 82 (05) :1012-1015
[9]   Determination of atomic site susceptibility tensors from polarized neutron diffraction data [J].
Gukasov, A ;
Brown, PJ .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2002, 14 (38) :8831-8839
[10]  
GUKASOV A, 2007, PHYSICA AMSTERDAM B, V397