1% solar cells derived from ultrathin carbon nanotube photoabsorbing films

被引:78
作者
Shea, Matthew J. [1 ]
Arnold, Michael S. [1 ]
机构
[1] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA
关键词
OPTICAL-PROPERTIES; ELECTRODES; PHOTODETECTORS; PHOTOVOLTAICS; SCAFFOLDS;
D O I
10.1063/1.4811359
中图分类号
O59 [应用物理学];
学科分类号
摘要
Using a carbon nanotube photoabsorbing film <5 nm in thickness, we demonstrate a 1% solar cell. Specifically, polymer wrapped, highly monochiral (7, 5) nanotubes are implemented in a bilayered heterojunction with acceptor C-60. The nanotubes drive 63% of the conversion, several times stronger than previously demonstrated. Peak external quantum efficiency (QE) of 43% at the nanotube bandgap (1055 nm) and power conversion efficiency of 0.95% and 1.02% at 1.0 and 1.5 suns, respectively, are achieved. The high internal QE from the ultrathin layers suggests that nanostructured or multijunction cells exploiting multiple nanotube layers will be many times more efficient. (C) 2013 AIP Publishing LLC.
引用
收藏
页数:5
相关论文
共 25 条
[1]   Environment Effects on Excitons in Semiconducting Carbon Nanotubes [J].
Ando, Tsuneya .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2010, 79 (02)
[2]   Broad Spectral Response Using Carbon Nanotube/Organic Semiconductor/C60 Photodetectors [J].
Arnold, Michael S. ;
Zimmerman, Jeramy D. ;
Renshaw, Christopher K. ;
Xu, Xin ;
Lunt, Richard R. ;
Austin, Christine M. ;
Forrest, Stephen R. .
NANO LETTERS, 2009, 9 (09) :3354-3358
[3]   Enhancing extraction of photogenerated excitons from semiconducting carbon nanotube films as photocurrent [J].
Bindl, Dominick J. ;
Shea, Matthew J. ;
Arnold, Michael S. .
CHEMICAL PHYSICS, 2013, 413 :29-34
[4]   Efficient Exciton Relaxation and Charge Generation in Nearly Monochiral (7,5) Carbon Nanotube/C60 Thin-Film Photovoltaics [J].
Bindl, Dominick J. ;
Arnold, Michael S. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2013, 117 (05) :2390-2395
[5]   Efficiently Harvesting Excitons from Electronic Type-Controlled Semiconducting Carbon Nanotube Films [J].
Bindl, Dominick J. ;
Wu, Meng-Yin ;
Prehn, Frederick C. ;
Arnold, Michael S. .
NANO LETTERS, 2011, 11 (02) :455-460
[6]   Dissociating Excitons Photogenerated in Semiconducting Carbon Nanotubes at Polymeric Photovoltaic Heterojunction Interfaces [J].
Bindl, Dominick J. ;
Safron, Nathaniel S. ;
Arnold, Michael S. .
ACS NANO, 2010, 4 (10) :5657-5664
[7]   Single-walled carbon nanotube scaffolds for dye-sensitized solar cells [J].
Brown, Patrick ;
Takechi, Kensuke ;
Kamat, Prashant V. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2008, 112 (12) :4776-4782
[8]   Extraordinary mobility in semiconducting carbon nanotubes [J].
Durkop, T ;
Getty, SA ;
Cobas, E ;
Fuhrer, MS .
NANO LETTERS, 2004, 4 (01) :35-39
[9]   Polymer-Free Near-Infrared Photovoltaics with Single Chirality (6,5) Semiconducting Carbon Nanotube Active Layers [J].
Jain, Rishabh M. ;
Howden, Rachel ;
Tvrdy, Kevin ;
Shimizu, Steven ;
Hilmer, Andrew J. ;
McNicholas, Thomas P. ;
Gleason, Karen K. ;
Strano, Michael S. .
ADVANCED MATERIALS, 2012, 24 (32) :4436-4439
[10]   Nanotube-Silicon Heterojunction Solar Cells [J].
Jia, Yi ;
Wei, Jinquan ;
Wang, Kunlin ;
Cao, Anyuan ;
Shu, Qinke ;
Gui, Xuchun ;
Zhu, Yanqiu ;
Zhuang, Daming ;
Zhang, Gong ;
Ma, Beibei ;
Wang, Liduo ;
Liu, Wenjin ;
Wang, Zhicheng ;
Luo, Jianbin ;
Wu, Dehai .
ADVANCED MATERIALS, 2008, 20 (23) :4594-4598