Antiferromagnetic properties in RFe2Ge2 (R=Tb,Dy,Ho)

被引:13
作者
Szytula, A
Baran, S
Leciejewicz, J
Penc, B
Stusser, N
Ding, YF
Zygmunt, A
Zukrowski, J
机构
[1] INST NUCL CHEM & TECHNOL,PL-03169 WARSAW,POLAND
[2] HAHN MEITNER INST BERLIN GMBH,BERLIN NEUTRON SCATTERING CTR,D-1000 BERLIN,GERMANY
[3] POLISH ACAD SCI,W TRZEBIATOWSKI INST LOW TEMP & STRUCT RES,PL-50950 WROCLAW,POLAND
[4] STANISLAW STASZIC UNIV MIN & MET,DEPT SOLID STATE PHYS,PL-30059 KRAKOW,POLAND
关键词
D O I
10.1088/0953-8984/9/32/002
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
X-ray and neutron diffraction measurements confirm that RFe2Ge2 (R = Tb, Dy and Ho) compounds show the tetragonal ThCr2Si2 type of crystal structure. Magnetization and magnetic susceptibility data indicate antiferromagnetic behaviour below the Neel temperatures at 8.5 K in TbFe2Ge2 and 3.35 K in DyFe2Ge2. A metamagnetic transition at H-c = 11 kOe and T = 4.2 K has been detected in TbFe2Ge2. The other two compounds give at 4.2 K magnetization curves characteristic for paramagnetic materials up to H = 50 kOe. The magnitudes of magnetic moments at H = 50 kOe are smaller than the free ion values for all three compounds. TbFe2Ge2 and DyFe2Ge2 exhibit at 1.5 K modulated antiferromagnetic order described by two component wavevectors k = \k(x), O, k(z)\. The magnetic moments are localized on the lanthanide ions and amount at 1.5 K to 7.68(11) and 7.3(3) mu(B) in TbFe2Ge2 and DyFe2Ge2 respectively. Diffuse magnetic peaks observed at 1.5 K in the neutron diffraction pattern of HoFe2Ge2 indicate that a long-range antiferromagnetic order starts to set up at this temperature.
引用
收藏
页码:6781 / 6789
页数:9
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