Activity of carbonaceous deposits in the selective reduction of nitrogen oxides

被引:17
作者
Connerton, J [1 ]
Joyner, RW [1 ]
Stockenhuber, M [1 ]
机构
[1] NOTTINGHAM TRENT UNIV,CATALYSIS RES LAB,NOTTINGHAM NG11 8NS,ENGLAND
关键词
D O I
10.1039/a606618f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Carbonaceous deposits, formed on the catalyst Cu/ZSM-5 by interaction at low temperature with propene, NO and oxygen, are characterised spectroscopically and shown to be able to carry out the selective catalytic reduction of NO; rates of reaction, which follow simple kinetics, are lower than in the absence of pre-deposited coke, and the results suggest an inverse correlation between catalyst Bronsted acidity and activity in NOx reduction.
引用
收藏
页码:185 / 186
页数:2
相关论文
共 14 条
[1]   MECHANISM OF THE LEAN NOX REACTION OVER CU/ZSM-5 [J].
ANSELL, GP ;
DIWELL, AF ;
GOLUNSKI, SE ;
HAYES, JW ;
RAJARAM, RR ;
TRUEX, TJ ;
WALKER, AP .
APPLIED CATALYSIS B-ENVIRONMENTAL, 1993, 2 (01) :81-100
[2]  
Aylor AW, 1996, STUD SURF SCI CATAL, V101, P661
[3]   Potential reaction paths in NOx reduction over Cu/ZSM-5 [J].
Beutel, T ;
Adelman, B ;
Sachtler, WMH .
CATALYSIS LETTERS, 1996, 37 (3-4) :125-130
[4]   INSITU FOURIER-TRANSFORM INFRARED-SPECTROSCOPY STUDY OF HY CRACKING CATALYSTS - COKE FORMATION AND THE NATURE OF THE ACTIVE-SITES [J].
BLACKMOND, DG ;
GOODWIN, JG ;
LESTER, JE .
JOURNAL OF CATALYSIS, 1982, 78 (01) :34-43
[5]   CHARACTERIZATION OF THE ACIDITY OF WELL-DEFINED CU-ZSM-5 CATALYSTS USING PYRIDINE AS A PROBE MOLECULE [J].
CONNERTON, J ;
JOYNER, RW ;
PADLEY, MB .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1995, 91 (12) :1841-1844
[6]  
GRUNERT W, 1994, J PHYS CHEM-US, V98, P10832
[7]   FORMATION, STORAGE AND REACTIVITY OF NITRILE SPECIES DURING THE LEAN NOX REACTION OVER CU/ZSM-5 CATALYSTS [J].
HAYES, NW ;
GRUNERT, W ;
HUTCHINGS, GJ ;
JOYNER, RW ;
SHPIRO, ES .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1994, (04) :531-532
[8]   Infrared spectroscopy studies of the mechanism of the selective reduction of NOx over Cu-ZSM-5 catalysts [J].
Hayes, NW ;
Joyner, RW ;
Shpiro, ES .
APPLIED CATALYSIS B-ENVIRONMENTAL, 1996, 8 (03) :343-363
[9]  
IWAMOTO M, 1990, STUD SURF SCI CATAL, V54, P121, DOI 10.1016/S0167-2991(08)60037-3
[10]   DETECTION OF SURFACE CN AND NCO SPECIES AS POSSIBLE REACTION INTERMEDIATES IN CATALYTIC LEAN NOX REDUCTION [J].
LI, C ;
BETHKE, KA ;
KUNG, HH ;
KUNG, MC .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1995, (08) :813-814