Quantum-mechanical models for photo-ionization: Uni-directional electron re-scattering by a laser pulse

The interaction of a hydrogen atom with a linearly (z-) polarized laser pulse is described by numerical solution of the three-dimensional Schrodinger equation. Photo-ionization of the ground state, with pulses having three or more optical cycles at photon energies well above the ionization potential and maximum intensity 10(15) W cm(-2), yields symmetric opposite fluxes of electrons preferentially in the +z and -z directions. One-cycle laser pulses can lead to modest symmetry breaking, e.g., more intense electron fluxes in the +z direction than in the -z direction, depending on the carrier-envelope phase (CEP) of the pulse. Production of uni-directional electron fluxes, similar to those observed in Coulomb scattering, calls for laser pulses with stronger intensity, or lower carrier frequency, or shorter duration with appropriate CEP, e.g., half-cycle pulses in the attosecond time domain. Here, uni-directionality is achieved by a four-step mechanism: (i) photo-ionization, (ii) turn-around of the electron, (iii) scattering from the atom's core and (iv) drift in the forward direction. (C) 2008 Elsevier B.V. All rights reserved.