Source apportionment of particulate matter in Europe: A review of methods and results

被引：783

作者：

Viana, M. ^{[1
,17
]}

Kuhlbusch, T. A. J. ^{[2
]}

Querol, X. ^{[1
,17
]}

Alastuey, A. ^{[1
,17
]}

Harrison, R. M. ^{[3
]}

Hopke, P. K. ^{[4
]}

Winiwarter, W. ^{[5
,6
]}

Vallius, A. ^{[7
]}

Szidat, S. ^{[8
]}

Prevot, A. S. H. ^{[9
]}

Hueglin, C. ^{[10
]}

Bloemen, H. ^{[11
]}

Wahlin, P. ^{[12
]}

Vecchi, R. ^{[13
]}

Miranda, A. I. ^{[18
]}

Kasper-Giebl, A. ^{[14
]}

Maenhaut, W. ^{[15
]}

Hitzenberger, R. ^{[16
]}

机构：

[1] Inst Environm Diag & Water Studies IDAEA CSIC, Barcelona, Spain

[2] IUTA eV, Duisburg, Germany

[3] Univ Birmingham, Sch Geog Earth & Environm Sci, Birmingham, W Midlands, England

[4] Clarkson Univ, Dept Chem & Biomol Engn, Potsdam, Germany

[5] ARC, Vienna, Austria

[6] Int Inst Appl Syst Anal, A-2361 Laxenburg, Austria

[7] Natl Publ Hlth Inst, Dept Environm Hlth, Kuopio, Finland

[8] Univ Bern, Dept Chem & Biochem, Bern, Switzerland

[9] Paul Scherrer Inst, Lab Atmospher Chem, Villigen, Switzerland

[10] Swiss Fed Labs Mat Testing & Res EMPA, Lab Air Pollut & Environm Technol, Dubendorf, Switzerland

[11] RIVM, Lab Milieumetingen, Bilthoven, Netherlands

[12] Aarhus Univ, NERI, Roskilde, Denmark

[13] Univ Milan, Inst Gen Appl Phys, Milan, Italy

[14] Vienna Univ Technol, Inst Chem Technol & Analyt, Aveiro, Portugal

[15] Univ Ghent, Inst Nucl Sci, Dept Analyt Chem, B-9000 Ghent, Belgium

[16] Univ Vienna, Vienna, Austria

[17] CSIC, Inst Earth Sci Jaume Almera, Barcelona, Spain

[18] Univ Aveiro, Dept Environm & Planning, P-3800 Aveiro, Portugal

来源：

JOURNAL OF AEROSOL SCIENCE | 2008年 / 39卷 / 10期

关键词：

PM10; PM2.5; Emission sources; Receptor modelling; Tracers; Research directions; Shipping emissions; Biomass burning;

D O I：

10.1016/j.jaerosci.2008.05.007

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

European publications dealing with source apportionment (SA) of atmospheric particulate matter (PM) between 1987 and 2007 were reviewed in the present work, with a focus on methods and results. The main goal of this meta-analysis was to provide a review of the most commonly used SA methods in Europe, their comparability and results, and to evaluate current trends and identify possible gaps of the methods and future research directions. Our analysis showed that studies throughout Europe agree on the identification of four main source types (PM10 and PM2.5): a vehicular source (traced by carbon/Fe/Ba/Zn/Cu), a crustal source (Al/Si/Ca/Fe), a sea-salt source (Na/Cl/Mg), and a mixed industrial/fuel-oil combustion (V/Ni/SO42-) and a secondary aerosol (SO42-/NO3-/NH4+) source (the latter two probably representing the same source type). Their contributions to bulk PM levels varied widely at different monitoring sites, and showed clear spatial patterns in the cases of the crustal and sea-salt sources. Other specific sources such as biomass combustion or shipping emissions were rarely identified, even though they may contribute significantly to PM levels in specific locations. (c) 2008 Elsevier Ltd. All rights reserved.

引用

页码：827 / 849

页数：23

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