Femtosecond time-resolved photoelectron imaging

被引:78
作者
Wang, L
Kohguchi, H
Suzuki, T [1 ]
机构
[1] Inst Mol Sci, Okazaki, Aichi 4448585, Japan
[2] Dalian Inst Chem Phys, Dalian, Peoples R China
来源
FARADAY DISCUSSIONS | 1999年 / 113卷
关键词
D O I
10.1039/a902866h
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Femtosecond time-resolved photoelectron imaging (FS-PEI) is presented for the first time. This novel method is tested with two-color photoionization of NO via the A 3s sigma state and applied to ultrafast dephasing in the intermediate case molecule pyrazine. The results illustrate the high-performance of FS-PEI in probing short-time dynamics in isolated molecules and clusters.
引用
收藏
页码:37 / 46
页数:10
相关论文
共 38 条
[1]   HIGH-RESOLUTION ANGLE-RESOLVED AND ENERGY-RESOLVED PHOTOELECTRON-SPECTROSCOPY OF NO - PARTIAL-WAVE DECOMPOSITION OF THE IONIZATION CONTINUUM [J].
ALLENDORF, SW ;
LEAHY, DJ ;
JACOBS, DC ;
ZARE, RN .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (04) :2216-2234
[2]  
BETHE HA, 1933, HDB PHYSIK, V24
[3]   Nonadiabatic dynamics in polyatomic systems studied by femtosecond time-resolved photoelectron spectroscopy [J].
Blanchet, V ;
Stolow, A .
JOURNAL OF CHEMICAL PHYSICS, 1998, 108 (11) :4371-4374
[4]   Photoelectron imaging spectrometry: Principle and inversion method [J].
Bordas, C ;
Paulig, F ;
Helm, H ;
Huestis, DL .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1996, 67 (06) :2257-2268
[5]   TWO-DIMENSIONAL IMAGING OF STATE-SELECTED PHOTODISSOCIATION PRODUCTS DETECTED BY MULTIPHOTON IONIZATION [J].
CHANDLER, DW ;
HOUSTON, PL .
JOURNAL OF CHEMICAL PHYSICS, 1987, 87 (02) :1445-1447
[6]   ANGULAR DISTRIBUTION OF PHOTOELECTRONS [J].
COOPER, J ;
ZARE, RN .
JOURNAL OF CHEMICAL PHYSICS, 1968, 48 (02) :942-&
[7]   Femtosecond time-resolved photoionization and photoelectron spectroscopy studies of ultrafast internal conversion in 1,3,5-hexatriene [J].
Cyr, DR ;
Hayden, CC .
JOURNAL OF CHEMICAL PHYSICS, 1996, 104 (02) :771-774
[8]   THE FAST COMPONENT IN THE DECAY OF PYRAZINE [J].
DELANGE, PJ ;
DRABE, KE ;
KOMMANDEUR, J .
JOURNAL OF CHEMICAL PHYSICS, 1986, 84 (01) :538-539
[9]   ROTATIONAL BRANCHING RATIOS IN (1+1) RESONANT-ENHANCED MULTIPHOTON IONIZATION OF NO VIA THE ALPHA-2-SIGMA+ STATE [J].
DIXIT, SN ;
LYNCH, DL ;
MCKOY, V ;
HUO, WM .
PHYSICAL REVIEW A, 1985, 32 (02) :1267-1270
[10]   Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen [J].
Eppink, ATJB ;
Parker, DH .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1997, 68 (09) :3477-3484