Carbon nanotube supported Pd catalyst for liquid-phase hydrodehalogenation of bromobenzene

被引：32

作者：

Chen, Long ^{[1
,2
]}

Yang, Keli ^{[1
,2
]}

Liu, Haitao ^{[1
,2
]}

Wang, Xiaolai ^{[1
]}

机构：

[1] Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Oxo Synth & Select Oxidat, Lanzhou 730000, Peoples R China

[2] Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China

来源：

CARBON | 2008年 / 46卷 / 15期

关键词：

D O I：

10.1016/j.carbon.2008.09.049

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

A multi-walled carbon nanotube (MWCNT) supported Pd catalyst has been prepared by conventional impregnation for the liquid-phase hydrodehalogenation of bromobenzene under mild reaction conditions. Compared with conventional supports such as activated carbon, Al2O3, SiO2 and MgO, MWCNTs as a catalyst support offer not only better performance but also a substantial reduction in the amount of Pd required. (C) 2008 Elsevier Ltd. All rights reserved.

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收藏

页码：2137 / 2139

页数：3

相关论文

共 8 条

[1] Catalytic hydrodechlorination over Pd supported on amorphous and structured carbon [J].

Amorim, C ;

Yuan, G ;

Patterson, PM ;

Keane, MA .

JOURNAL OF CATALYSIS, 2005, 234 (02) :268-281

[2] Pd/C-catalyzed transfer reduction of aryl chlorides with sodium formate in water [J].

Arcadi, A ;

Cerichelli, G ;

Chiarini, M ;

Vico, R ;

Zorzan, D .

EUROPEAN JOURNAL OF ORGANIC CHEMISTRY, 2004, 2004 (16) :3404-3407

[3] Hydrodechlorination of 4-chlorophenol in aqueous phase using Pd/AC catalysts prepared with modified active carbon supports [J].

Calvo, L. ;

Gilarranz, M. A. ;

Casas, J. A. ;

Mohedano, A. F. ;

Rodriguez, J. J. .

APPLIED CATALYSIS B-ENVIRONMENTAL, 2006, 67 (1-2) :68-76

[4] Treatment of chlorophenols-bearing wastewaters through hydrodechlorination using Pd/activated carbon catalysts [J].

Calvo, L ;

Mohedano, AF ;

Casas, JA ;

Gilarranz, MA ;

Rodríguez, JJ .

CARBON, 2004, 42 (07) :1377-1381

[5]

CHEN L, MATER CHEM PHYS, DOI DOI 10.1016/I.MATCHEM2HYS.2008.05.081

[6] Spontaneous reduction of metal ions on the sidewalls of carbon nanotubes [J].

Choi, HC ;

Shim, M ;

Bangsaruntip, S ;

Dai, HJ .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2002, 124 (31) :9058-9059

[7] Bimetallic catalysis on carbon nanotubes for the selective hydrogenation of cinnamaldehyde [J].

Vu, Hung ;

Goncalves, Filomena ;

Philippe, Regis ;

Lamouroux, Emmanuel ;

Corrias, Massimiliano ;

Kihn, Yolande ;

Plee, Dominique ;

Kalck, Philippe ;

Serp, Philippe .

JOURNAL OF CATALYSIS, 2006, 240 (01) :18-22

[8] Synthesis and electrochemical characterization of uniformly-dispersed high loading Pt nanoparticles on sonochemically-treated carbon nanotubes [J].

Xing, YC .

JOURNAL OF PHYSICAL CHEMISTRY B, 2004, 108 (50) :19255-19259