The North Atlantic Marine Boundary Layer Experiment (NAMBLEX). Overview of the campaign held at Mace Head, Ireland, in summer 2002

被引:47
作者
Heard, D. E. [1 ]
Read, K. A.
Methven, J.
Al-Haider, S.
Bloss, W. J.
Johnson, G. P.
Pilling, M. J.
Seakins, P. W.
Smith, S. C.
Sommariva, R.
Stanton, J. C.
Still, T. J.
Ingham, T.
Brooks, B.
De Leeuw, G.
Jackson, A. V.
McQuaid, J. B.
Morgan, R.
Smith, M. H.
Carpenter, L. J.
Carslaw, N.
Hamilton, J.
Hopkins, J. R.
Lee, J. D.
Lewis, A. C.
Purvis, R. M.
Wevill, D. J.
Brough, N.
Green, T.
Mills, G.
Penkett, S. A.
Plane, J. M. C.
Saiz-Lopez, A.
Worton, D.
Monks, P. S.
Fleming, Z.
Rickard, A. R.
Alfarra, M. R.
Allan, J. D.
Bower, K.
Coe, H.
Cubison, M.
Flynn, M.
McFiggans, G.
Gallagher, M.
Norton, E. G.
O'Dowd, C. D.
Shillito, J.
Topping, D.
Vaughan, G.
机构
[1] Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England
[2] Univ Reading, Dept Meteorol, Reading RG6 6AH, Berks, England
[3] Univ Leeds, Sch Earth & Environm, Leeds LS2 9JT, W Yorkshire, England
[4] Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England
[5] Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England
[6] Univ Leicester, Dept Chem, Leicester LE1 7RH, Leics, England
[7] Univ Manchester, SEAES, Manchester M60 1QD, Lancs, England
[8] Univ Cambridge, Chem Lab, Cambridge CB2 1EW, England
[9] Univ Bristol, Sch Chem, Bristol BS8 1TH, Avon, England
[10] Univ Birmingham, Sch Geog Earth & Environm Sci, Dept Phys, Birmingham B15 2TT, W Midlands, England
[11] Univ Edinburgh, Sch Chem, Edinburgh EH9 3JJ, Midlothian, Scotland
[12] Natl Univ Ireland Galway, Galway, Ireland
[13] TNO, NL-2509 JG The Hague, Netherlands
[14] Cranfield Univ, Facil Airborne Atmospher Measurement, Cranfield MK43 0AL, Beds, England
基金
英国自然环境研究理事会;
关键词
D O I
10.5194/acp-6-2241-2006
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The North Atlantic Marine Boundary Layer Experiment ( NAMBLEX), involving over 50 scientists from 12 institutions, took place at Mace Head, Ireland (53.32 degrees N, 9.90 degrees W), between 23 July and 4 September 2002. A wide range of state-of-the-art instrumentation enabled detailed measurements of the boundary layer structure and atmospheric composition in the gas and aerosol phase to be made, providing one of the most comprehensive in situ studies of the marine boundary layer to date. This overview paper describes the aims of the NAMBLEX project in the context of previous field campaigns in the Marine Boundary Layer ( MBL), the overall layout of the site, a summary of the instrumentation deployed, the temporal coverage of the measurement data, and the numerical models used to interpret the field data. Measurements of some trace species were made for the first time during the campaign, which was characterised by predominantly clean air of marine origin, but more polluted air with higher levels of NOx originating from continental regions was also experienced. This paper provides a summary of the meteorological measurements and Planetary Boundary Layer ( PBL) structure measurements, presents time series of some of the longer-lived trace species ( O-3, CO, H-2, DMS, CH4 , NMHC, NOx, NOy, PAN) and summarises measurements of other species that are described in more detail in other papers within this special issue, namely oxygenated VOCs, HCHO, peroxides, organo-halogenated species, a range of shorter lived halogen species ( I-2, OIO, IO, BrO), NO3 radicals, photolysis frequencies, the free radicals OH, HO2 and ( HO2 + Sigma RO2), as well as a summary of the aerosol measurements. NAMBLEX was supported by measurements made in the vicinity of Mace Head using the NERC Dornier-228 aircraft. Using ECMWF windfields, calculations were made of the air-mass trajectories arriving at Mace Head during NAMBLEX, and were analysed together with both meteorological and trace-gas measurements. In this paper a chemical climatology for the duration of the campaign is presented to interpret the distribution of air-mass origins and emission sources, and to provide a convenient framework of air-mass classification that is used by other papers in this issue for the interpretation of observed variability in levels of trace gases and aerosols.
引用
收藏
页码:2241 / 2272
页数:32
相关论文
共 83 条
[1]   Observations of the nitrate radical in the marine boundary layer [J].
Allan, BJ ;
Carslaw, N ;
Coe, H ;
Burgess, RA ;
Plane, JMC .
JOURNAL OF ATMOSPHERIC CHEMISTRY, 1999, 33 (02) :129-154
[2]   Quantitative sampling using an Aerodyne aerosol mass spectrometer - 1. Techniques of data interpretation and error analysis [J].
Allan, JD ;
Jimenez, JL ;
Williams, PI ;
Alfarra, MR ;
Bower, KN ;
Jayne, JT ;
Coe, H ;
Worsnop, DR .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D3)
[3]   Evaluated kinetic, photochemical and heterogeneous data for atmospheric chemistry .5. IUPAC Subcommittee on Gas Kinetic Data Evaluation for Atmospheric Chemistry [J].
Atkinson, R ;
Baulch, DL ;
Cox, RA ;
Hampson, RF ;
Kerr, JA ;
Rossi, MJ ;
Troe, J .
JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 1997, 26 (03) :521-1011
[4]  
BAUGUITTE S, 2000, STUDY TOPOSPHERIC RE, P448
[5]   A broadband cavity ringdown spectrometer for in-situ measurements of atmospheric trace gases [J].
Bitter, M ;
Ball, SM ;
Povey, IM ;
Jones, RL .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2005, 5 :2547-2560
[6]  
Bloss WJ, 2005, GEOPHYS RES LETT, V32, DOI [10.1029/2004GL022084, 10.1029/2004GL022168]
[7]  
Brasseur G.P., 1999, Atmospheric Chemistry and Global Change
[8]  
BRASSEUR GP, 2002, IGBP SERIES
[9]   Intercomparison of aircraft instruments on board the C-130 and Falcon 20 over southern Germany during EXPORT 2000 [J].
Brough, N ;
Reeves, CE ;
Penkett, SA ;
Stewart, DJ ;
Dewey, K ;
Kent, J ;
Barjat, H ;
Monks, PS ;
Ziereis, H ;
Stock, P ;
Huntrieser, H ;
Schlager, H .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2003, 3 :2127-2138
[10]   The use of trajectory cluster analysis to interpret trace gas measurements at Mace Head, Ireland [J].
Cape, JN ;
Methven, J ;
Hudson, LE .
ATMOSPHERIC ENVIRONMENT, 2000, 34 (22) :3651-3663