Experimental investigation of ultra-fine particle size distribution near a busy road

被引:48
作者
Gramotnev, G [1 ]
Ristovski, Z [1 ]
机构
[1] Queensland Univ Technol, Sch Phys & Chem Sci, Int Lab Air Qual & Hlth, Brisbane, Qld 4001, Australia
关键词
ultra-fine particles; size distribution; busy road; particle formation; aerosol evolution;
D O I
10.1016/j.atmosenv.2003.12.028
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In this paper, evolution of the size distribution of fine and ultra-fine particles emitted from vehicles on a busy road is investigated experimentally. In particular, several different modes (distinct maxima) of the particle size distribution are investigated as a function of the distance from the road. An unusual and complex evolution of these modes is discovered. In particular, it is demonstrated that some of the modes tend to shift towards smaller particle size, which has never been reported previously. Complex correlation between the modes is determined experimentally. In addition, for the first time, the total number concentration is clearly shown to go through a significant maximum at some distance from the road. This could have significant influence on the assessment of exposure to fine and ultra-fine particles in the vicinity of busy roads. (C) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1767 / 1776
页数:10
相关论文
共 15 条
[1]   Observations of new particle formation in urban air [J].
Alam, A ;
Shi, JP ;
Harrison, RM .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D3)
[2]   CONTROLLED EXPOSURES OF VOLUNTEERS TO RESPIRABLE CARBON AND SULFURIC-ACID AEROSOLS [J].
ANDERSON, KR ;
AVOL, EL ;
EDWARDS, SA ;
SHAMOO, DA ;
PENG, RC ;
LINN, WS ;
HACKNEY, JD .
JOURNAL OF THE AIR & WASTE MANAGEMENT ASSOCIATION, 1992, 42 (06) :770-776
[3]  
Bowman AW, 1997, Applied Smoothing Techniques for Data Analysis: the Kernel Approach with S-Plus Illustrations
[4]   AN ASSOCIATION BETWEEN AIR-POLLUTION AND MORTALITY IN 6 UNITED-STATES CITIES [J].
DOCKERY, DW ;
POPE, CA ;
XU, XP ;
SPENGLER, JD ;
WARE, JH ;
FAY, ME ;
FERRIS, BG ;
SPEIZER, FE .
NEW ENGLAND JOURNAL OF MEDICINE, 1993, 329 (24) :1753-1759
[5]  
GRAMOTNEV DK, UNPUB NEW MECH AEROS
[6]   Determination of average emission factors for vehicles on a busy road [J].
Gramotnev, G ;
Brown, R ;
Ristovski, Z ;
Hitchins, J ;
Morawska, L .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (04) :465-474
[7]  
GRAMOTNEV G, IN PRESS ATMOSPHERIC, DOI DOI 10.1016/J.ATMOSENV.2004.02.015
[8]   Concentrations of submicrometre particles from vehicle emissions near a major road [J].
Hitchins, J ;
Morawska, L ;
Wolff, R ;
Gilbert, D .
ATMOSPHERIC ENVIRONMENT, 2000, 34 (01) :51-59
[9]  
Larsen R.J., 2001, INTRO MATH STAT ITS, V3rd
[10]  
Ripley B.D., 2000, MODERN APPL STAT S P