Anticorrelation between ferromagnetism and ferroelectricity in perovskite manganites

被引:93
作者
Goto, T [1 ]
Yamasaki, Y
Watanabe, H
Kimura, T
Tokura, Y
机构
[1] Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan
[2] Bell Labs, Lucent Technol, Murray Hill, NJ 07974 USA
[3] ERATO, SSS, JST Agcy, Tsukuba, Ibaraki 3058562, Japan
[4] CERC, Natl Inst AIST, Tsukuba, Ibaraki 3058562, Japan
关键词
D O I
10.1103/PhysRevB.72.220403
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Magnetic and dielectric properties have been investigated for a mixed-crystal system Tb1-xGdxMnO3 in between TbMnO3 with ferroelectric and incommensurate antiferromagnetic (AFM) orders and GdMnO3 with paraelectric and canted AFM (weakly ferromagnetic) states, as functions of x, temperature T, and magnetic field B applied along the c axis. A systematic study on the magnetic and electric phase diagrams in the x-T, B-T, and x-B planes has revealed important interplay between Mn d-electron spins and Gd f-electron moments. A clear anticorrelation between the (weak) ferromagnetism and the ferroelectricity is observed near the phase boundaries.
引用
收藏
页数:4
相关论文
共 16 条
[1]   Magnetic-field-induced transition in the lattice modulation of colossal magnetoelectric GdMnO3 and TbMnO3 compounds -: art. no. 100102 [J].
Arima, T ;
Goto, T ;
Yamasaki, Y ;
Miyasaka, S ;
Ishii, K ;
Tsubota, M ;
Inami, T ;
Murakami, Y ;
Tokura, Y .
PHYSICAL REVIEW B, 2005, 72 (10)
[2]   Revival of the magnetoelectric effect [J].
Fiebig, M .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2005, 38 (08) :R123-R152
[3]   Complex interplay of 3d and 4f magnetism in La1-xGdxMnO3 -: art. no. 024414 [J].
Hemberger, J ;
Lobina, S ;
von Nidda, HAK ;
Tristan, N ;
Ivanov, VY ;
Mukhin, AA ;
Balbashov, AM ;
Loidl, A .
PHYSICAL REVIEW B, 2004, 70 (02) :024414-1
[4]  
KADOMTSEVA AM, 2005, JETP LETT, V81, P22
[5]   Magnetic structure of TbMnO3 by neutron diffraction -: art. no. 012401 [J].
Kajimoto, R ;
Yoshizawa, H ;
Shintani, H ;
Kimura, T ;
Tokura, Y .
PHYSICAL REVIEW B, 2004, 70 (01) :012401-1
[6]   Magnetic structure of TbMnO3 by neutron diffraction (vol B 70, art no 012401, 2004) -: art. no. 219904 [J].
Kajimoto, R ;
Yoshizawa, H ;
Shintani, H ;
Kimura, T ;
Tokura, Y .
PHYSICAL REVIEW B, 2004, 70 (21)
[7]   Magnetic inversion symmetry breaking and ferroelectricity in TbMnO3 -: art. no. 087206 [J].
Kenzelmann, M ;
Harris, AB ;
Jonas, S ;
Broholm, C ;
Schefer, J ;
Kim, SB ;
Zhang, CL ;
Cheong, SW ;
Vajk, OP ;
Lynn, JW .
PHYSICAL REVIEW LETTERS, 2005, 95 (08)
[8]   Magnetoelectric phase diagrams of orthorhombic RMnO3 (R=Gd, Tb, and Dy) [J].
Kimura, T ;
Lawes, G ;
Goto, T ;
Tokura, Y ;
Ramirez, AP .
PHYSICAL REVIEW B, 2005, 71 (22)
[9]   Distorted perovskite with eg1 configuration as a frustrated spin system -: art. no. 060403 [J].
Kimura, T ;
Ishihara, S ;
Shintani, H ;
Arima, T ;
Takahashi, KT ;
Ishizaka, K ;
Tokura, Y .
PHYSICAL REVIEW B, 2003, 68 (06)
[10]   Magnetic control of ferroelectric polarization [J].
Kimura, T ;
Goto, T ;
Shintani, H ;
Ishizaka, K ;
Arima, T ;
Tokura, Y .
NATURE, 2003, 426 (6962) :55-58