A laboratory study of agricultural crop residue combustion in China: Emission factors and emission inventory

被引:202
作者
Zhang, Hefeng [1 ]
Ye, Xingnan [1 ]
Cheng, Tiantao [1 ]
Chen, Jianmin [1 ]
Yang, Xin [1 ]
Wang, Lin [2 ]
Zhang, Renyi [2 ]
机构
[1] Fudan Univ, Dept Environm Sci & Engn, Ctr Atmospher Chem Studies, Shanghai 200433, Peoples R China
[2] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA
基金
中国国家自然科学基金;
关键词
Agricultural crop residue; Gaseous pollutant; Emission factor; Emission inventory; Emission allocation;
D O I
10.1016/j.atmosenv.2008.08.015
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The burning of agricultural crop residue represents a major source of trace gases (CO, CO2, NO, NO2, and NOx) and particulate matter on a regional and global scale. This study investigates the gaseous and particulate emissions from the burning of rice, wheat and corn straws, which are three major agricultural crop residues in China, using a self-built burning stove and an aerosol chamber. Emission factors Of CO2, CO, NO, NO2 and NOx were measured to be 791.3, 64.2,1.02, 0.79 and 1.81 g kg(-1) for rice straw, 1557.9,141.2, 0.79, 0.32 and 1.12 g kg(-1) for wheat straw, and 1261.5, 114.7, 0.85, 0.43 and 1.28 g kg(-1) for corn straw, respectively. The corresponding emission factors of particle number are 1.8 X 10(13), 1.0 x 10(13), and 1.7 x 10(13) particles kg(-1), respectively. The total emissions of CO, CO2, and NOx from rice, wheat and corn straw burnings in China for the year 2004 were estimated to be 22.59, 252.92, and 0.28 Tg, respectively. The percentages of CO, CO2, and NOx to the total emissions were 13.9%, 15.3%, and 31.4% for rice straw, 32.9%, 32.5%, and 20.9% for wheat straw, and 53.2%, 52.2%, and 47.6% for corn straw, respectively. In addition, the emission allocations of agricultural crop residue burning were also plotted in different regions of China using a simple geographic information system (GIS). (c) 2008 Elsevier Ltd. All rights reserved.
引用
收藏
页码:8432 / 8441
页数:10
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