Angle-resolved photoemission spectroscopy of the insulating NaxWO3:: Anderson localization, polaron formation, and remnant Fermi surface -: art. no. 147603

被引:33
作者
Raj, S [1 ]
Hashimoto, D
Matsui, H
Souma, S
Sato, T
Takahashi, T
Sarma, DD
Mahadevan, P
Oishi, S
机构
[1] Tohoku Univ, Dept Phys, Sendai, Miyagi 9808578, Japan
[2] JST, CREST, Kawaguchi 3320012, Japan
[3] Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India
[4] SN Bose Natl Ctr Basic Sci, Kolkata 700098, W Bengal, India
[5] Shinshu Univ, Fac Engn, Nagano 3808553, Japan
关键词
D O I
10.1103/PhysRevLett.96.147603
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The electronic structure of the insulating sodium tungsten bronze, Na0.025WO3, is investigated by high-resolution angle-resolved photoemission spectroscopy. We find that near-E-F states are localized due to the strong disorder arising from random distribution of Na+ ions in the WO3 lattice, which makes the system insulating. The temperature dependence of photoemission spectra provides direct evidence for polaron formation. The remnant Fermi surface of the insulator is found to be the replica of the real Fermi surface in the metallic system.
引用
收藏
页数:4
相关论文
共 32 条
[1]   ABSENCE OF DIFFUSION IN CERTAIN RANDOM LATTICES [J].
ANDERSON, PW .
PHYSICAL REVIEW, 1958, 109 (05) :1492-1505
[2]   THE ANDERSON-MOTT TRANSITION [J].
BELITZ, D ;
KIRKPATRICK, TR .
REVIEWS OF MODERN PHYSICS, 1994, 66 (02) :261-390
[3]   VACUUM ULTRAVIOLET-PHOTOEMISSION STUDY OF SOME SODIUM TUNGSTEN BRONZES, NAX WO3 [J].
BENBOW, RL ;
HURYCH, Z .
PHYSICAL REVIEW B, 1978, 17 (12) :4527-4536
[4]   PHYSICAL INTERPRETATION OF WEAK LOCALIZATION - A TIME-OF-FLIGHT EXPERIMENT WITH CONDUCTION ELECTRONS [J].
BERGMANN, G .
PHYSICAL REVIEW B, 1983, 28 (06) :2914-2920
[5]   WEAK LOCALIZATION IN THIN-FILMS - A TIME-OF-FLIGHT EXPERIMENT WITH CONDUCTION ELECTRONS [J].
BERGMANN, G .
PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 1984, 107 (01) :1-58
[6]   PROJECTOR AUGMENTED-WAVE METHOD [J].
BLOCHL, PE .
PHYSICAL REVIEW B, 1994, 50 (24) :17953-17979
[7]   NUMERICAL-CALCULATION OF PATH-INTEGRALS - THE SMALL-POLARON MODEL [J].
DERAEDT, H ;
LAGENDIJK, A .
PHYSICAL REVIEW B, 1983, 27 (10) :6097-6109
[8]   EVIDENCE FOR POLARONIC STATES IN NA0.1WO3 FROM RAMAN-SCATTERING [J].
EGDELL, RG ;
JONES, GB .
JOURNAL OF SOLID STATE CHEMISTRY, 1989, 81 (01) :137-141
[9]   THE SODIUM TUNGSTEN BRONZES - A STUDY OF THE CHANGES IN ELECTRONIC-STRUCTURE WITH COMPOSITION USING HIGH-RESOLUTION ELECTRON-SPECTROSCOPY [J].
HILL, MD ;
EGDELL, RG .
JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 1983, 16 (32) :6205-6220
[10]   METAL-NONMETAL TRANSITION IN TUNGSTEN BRONZES - A PHOTOEMISSION-STUDY [J].
HOLLINGER, G ;
PERTOSA, P ;
DOUMERC, JP ;
HIMPSEL, FJ ;
REIHL, B .
PHYSICAL REVIEW B, 1985, 32 (04) :1987-1991