Field-free molecular orientation by an intense nonresonant two-color laser field with a slow turn on and rapid turn off

被引:91
作者
Muramatsu, Masahiro [1 ]
Hita, Masafumi [1 ]
Minemoto, Shinichirou [1 ]
Sakai, Hirofumi [1 ]
机构
[1] Univ Tokyo, Grad Sch Sci, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan
来源
PHYSICAL REVIEW A | 2009年 / 79卷 / 01期
基金
日本学术振兴会;
关键词
fluorine compounds; molecular orientation; molecule-photon collisions; polarisability; quantum optics; radiation pressure; rotational states; POLARIZABILITY; STATES;
D O I
10.1103/PhysRevA.79.011403
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We propose a practical and versatile technique to achieve completely field-free molecular orientation with an intense, nonresonant, two-color laser field with a slow turn on and rapid turn off. The technique is based on the combined effects of both anisotropic polarizability interaction and anisotropic hyperpolarizability interaction. Using a FCN molecule as a sample, we show that the orientation achieved adiabatically by the peak of the laser pulse can be successfully revived at the rotational period of the molecule with the same degree of orientation. The crucial importance of the sufficiently slow turn on of the laser pulse is emphasized to achieve the highest possible degree of orientation.
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页数:4
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