High-yield dielectrophoretic assembly of two-dimensional graphene nanostructures

被引:37
作者
Burg, Brian R. [1 ]
Luetolf, Fabian [1 ]
Schneider, Julian [1 ]
Schirmer, Niklas C. [1 ]
Schwamb, Timo [1 ]
Poulikakos, Dimos [1 ]
机构
[1] ETH, Lab Thermodynam Emerging Technol, Dept Mech & Proc Engn, CH-8092 Zurich, Switzerland
关键词
coating techniques; electrical resistivity; electrodes; electrophoresis; graphene; sheet materials; thick films; INDIVIDUAL CARBON NANOTUBES; OXIDE; TRANSPARENT; DEPOSITION; FILMS; SEPARATION; SHEETS;
D O I
10.1063/1.3077197
中图分类号
O59 [应用物理学];
学科分类号
摘要
Graphene handling is still dominated by serial mechanical exfoliation, which may well facilitate measurements in a laboratory environment but does not allow reliable larger-scale integration. Herein we demonstrate the controlled, high-yield (>90%), site-selective deposition of ultrathin few-layer (three to ten) graphene oxide by dielectrophoresis between prefabricated electrodes. Individual layers are found near the edges. Initially insulating, thermal reduction at 450 degrees C thins out the two-dimensional few-atom thick films and dramatically reduces electrical resistances down to 40 k Omega. Conductivities between 15 and 36 S/cm are obtained. The introduced method permits the nonintrusive, parallel, large-scale assembly of soluble two-dimensional nanostructures and sheets.
引用
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页数:3
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