Surface-enhanced Raman spectroscopy for trace arsenic detection in contaminated water

被引:260
作者
Mulvihill, Martin [1 ]
Tao, Andrea [2 ]
Benjauthrit, Kanokraj [1 ]
Arnold, John [1 ]
Yang, Peidong [1 ]
机构
[1] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
[2] Univ Calif Santa Barbara, Inst Collaborat Biotechnol, Santa Barbara, CA 93106 USA
关键词
arsenic; Raman spectroscopy; silver; surface effects; water analysis;
D O I
10.1002/anie.200800776
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
(Graph Presented) Getting to the bottom of groundwater: The development of a reliable, portable, and simple-to-use device for detecting arsenic in groundwater is urgently needed in developing nations such as Bangladesh, where contaminated groundwater is at the root of a public health crisis. Toward this end, a highly sensitive platform utilizing surface-enhanced Raman spectroscopy (SERS, see picture) is used to quantitatively detect arsenate in water down to 1 ppb. © 2008 Wiley-VCH Verlag GmbH & Co. KGaA.
引用
收藏
页码:6456 / 6460
页数:5
相关论文
共 30 条
[1]   Tunable plasmonic response from alkanethiolate-stabilized gold nanoparticle superlattices: Evidence of near-field coupling [J].
Chen, Chi-Fan ;
Tzeng, Shien-Der ;
Chen, Hung-Ying ;
Lin, Kuan-Jiuh ;
Gwo, Shangjr .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2008, 130 (03) :824-+
[2]   PLASMA RESONANCE ENHANCEMENT OF RAMAN-SCATTERING BY PYRIDINE ADSORBED ON SILVER OR GOLD SOL PARTICLES OF SIZE COMPARABLE TO THE EXCITATION WAVELENGTH [J].
CREIGHTON, JA ;
BLATCHFORD, CG ;
ALBRECHT, MG .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS II, 1979, 75 :790-798
[3]   Development of a compact, handheld Raman instrument with no moving parts for use in field analysis [J].
Cullum, BM ;
Mobley, J ;
Chi, ZH ;
Stokes, DL ;
Miller, GH ;
Vo-Dinh, T .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2000, 71 (04) :1602-1607
[4]   Detection of arsenic in groundwater using a surface plasmon resonance sensor [J].
Forzani, Erica S. ;
Foley, Kyle ;
Westerhoff, Paul ;
Tao, Nongjian .
SENSORS AND ACTUATORS B-CHEMICAL, 2007, 123 (01) :82-88
[5]   Raman spectroscopy of selected arsenates - implications for soil remediation [J].
Frost, RL ;
Kloprogge, T ;
Weier, ML ;
Martens, WN ;
Ding, Z ;
Edwards, HGH .
SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY, 2003, 59 (10) :2241-2246
[6]   SURFACE-ENHANCED RAMAN-SCATTERING (SERS) FROM SILVER COLLOIDS OF VANADATE, PHOSPHATE AND ARSENATE [J].
GREAVES, SJ ;
GRIFFITH, WP .
JOURNAL OF RAMAN SPECTROSCOPY, 1988, 19 (08) :503-507
[7]  
HARRIS D, 2002, QUANTITATIVE CHEM AN, P88
[8]   Ultrafast electron relaxation dynamics in coupled metal nanoparticles in aggregates [J].
Jain, PK ;
Qian, W ;
El-Sayed, MA .
JOURNAL OF PHYSICAL CHEMISTRY B, 2006, 110 (01) :136-142
[9]   Universal scaling of plasmon coupling in metal nanostructures: Extension from particle pairs to nanoshells [J].
Jain, Prashant K. ;
El-Sayed, Mostafa A. .
NANO LETTERS, 2007, 7 (09) :2854-2858
[10]   SURFACE RAMAN SPECTROELECTROCHEMISTRY .1. HETEROCYCLIC, AROMATIC, AND ALIPHATIC-AMINES ADSORBED ON ANODIZED SILVER ELECTRODE [J].
JEANMAIRE, DL ;
VANDUYNE, RP .
JOURNAL OF ELECTROANALYTICAL CHEMISTRY, 1977, 84 (01) :1-20