Trans-Pacific dust events observed at Whistler, British Columbia during INTEX-B

被引:49
作者
McKendry, I. G. [1 ]
Macdonald, A. M. [2 ]
Leaitch, W. R. [2 ]
van Donkelaar, A. [3 ]
Zhang, Q. [4 ]
Duck, T. [3 ]
Martin, R. V. [3 ]
机构
[1] Univ British Columbia, Dept Geog, Vancouver, BC V6T 1Z2, Canada
[2] Environm Canada, Sci & Technol Branch, Toronto, ON M3H 5T4, Canada
[3] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS M3J 1P3, Canada
[4] SUNY Albany, New York, NY USA
基金
加拿大自然科学与工程研究理事会;
关键词
D O I
10.5194/acp-8-6297-2008
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The meteorology and physico-chemical characteristics of aerosol associated with two new cases of long range dust transport affecting western Canada during spring 2006 are described. Each event showed enhancements of both sulfate aerosol and crustal material of Asian origin. However, the events were of quite different character and demonstrate the highly variable nature of such events. The April event was a significant dust event with considerable enhancement of fine particle sulfate while the May event was a weaker dust event, also with significant fine particle sulfate enhancement. The latter event was notable in the sense that it was of short duration and was quickly followed by a large increase of organic material likely of regional origin. Comparison of these two events with other documented cases extending back to 1993, suggests that all dust events show coincident enhancements of sulfate and crustal aerosol. However, events vary across a wide continuum based on the magnitude of aerosol enhancements and their sulfate to calcium ratios. At one extreme, events are dominated by highly significant crustal enhancements (e.g. the well-documented 1998 and 2001 'dust' events) while at the other are events with some dust transport, but where sulfate enhancements are of very high magnitude (e.g. the 1993 event at Crater Lake and the 15 May 2006 event at Whistler). Other events represent a 'mix'. It is likely that this variability is a function of the comparative strengths of the dust and anthropogenic SO2 sources, the transport pathway and in particular the extent to which dust is transported across industrial SO2 sources, and finally, meteorological and chemical processes.
引用
收藏
页码:6297 / 6307
页数:11
相关论文
共 44 条
[1]   Particle characteristics following cloud-modified transport from Asia to North America -: art. no. D23S26 [J].
Brock, CA ;
Hudson, PK ;
Lovejoy, ER ;
Sullivan, A ;
Nowak, JB ;
Huey, LG ;
Cooper, OR ;
Cziczo, DJ ;
de Gouw, J ;
Fehsenfeld, FC ;
Holloway, JS ;
Hübler, G ;
Lafleur, BG ;
Murphy, DM ;
Neuman, JA ;
Nicks, DK ;
Orsini, DA ;
Parrish, DD ;
Ryerson, TB ;
Tanner, DJ ;
Warneke, C ;
Weber, RJ ;
Wilson, JC .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D23) :1-17
[2]   Intercontinental transport of pollution and dust aerosols: implications for regional air quality [J].
Chin, Mian ;
Diehl, T. ;
Ginoux, P. ;
Malm, W. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (21) :5501-5517
[3]   A case study of transpacific warm conveyor belt transport:: Influence of merging airstreams on trace gas import to North America -: art. no. D23S08 [J].
Cooper, OR ;
Forster, C ;
Parrish, D ;
Trainer, M ;
Dunlea, E ;
Ryerson, T ;
Hübler, G ;
Fehsenfeld, F ;
Nicks, D ;
Holloway, J ;
de Gouw, J ;
Warneke, C ;
Roberts, JM ;
Flocke, F ;
Moody, J .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2004, 109 (D23) :1-17
[4]   Transport of forest fire emissions from Alaska and the Yukon Territory to Nova Scotia during summer 2004 [J].
Duck, Thomas J. ;
Firanski, Bernard J. ;
Millet, Dylan B. ;
Goldstein, Allen H. ;
Allan, James ;
Holzinger, Rupert ;
Worsnop, Douglas R. ;
White, Allen B. ;
Stohl, Andreas ;
Dickinson, Cameron S. ;
van Donkelaar, Aaron .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2007, 112 (D10)
[5]   Evolution of Asian aerosols during transpacific transport in INTEX-B [J].
Dunlea, E. J. ;
DeCarlo, P. F. ;
Aiken, A. C. ;
Kimmel, J. R. ;
Peltier, R. E. ;
Weber, R. J. ;
Tomlinson, J. ;
Collins, D. R. ;
Shinozuka, Y. ;
McNaughton, C. S. ;
Howell, S. G. ;
Clarke, A. D. ;
Emmons, L. K. ;
Apel, E. C. ;
Pfister, G. G. ;
van Donkelaar, A. ;
Martin, R. V. ;
Millet, D. B. ;
Heald, C. L. ;
Jimenez, J. L. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2009, 9 (19) :7257-7287
[6]   The impact of transpacific transport of mineral dust in the United States [J].
Fairlie, T. Duncan ;
Jacob, Daniel J. ;
Park, Rokjin J. .
ATMOSPHERIC ENVIRONMENT, 2007, 41 (06) :1251-1266
[7]   A simulated climatology of Asian dust aerosol and its trans-Pacific transport. Part II: Interannual variability and climate connections [J].
Gong, SL ;
Zhang, XY ;
Zhao, TL ;
Zhang, XB ;
Barrie, LA ;
McKendry, IG ;
Zhao, CS .
JOURNAL OF CLIMATE, 2006, 19 (01) :104-122
[8]  
Hacker JP, 2001, J APPL METEOROL, V40, P1617, DOI 10.1175/1520-0450(2001)040<1617:MDTOAP>2.0.CO
[9]  
2
[10]   Transpacific transport of Asian anthropogenic aerosols and its impact on surface air quality in the United States [J].
Heald, Colette L. ;
Jacob, Daniel J. ;
Park, Rokjin J. ;
Alexander, Becky ;
Fairlie, T. Duncan ;
Yantosca, Robert M. ;
Chu, D. Allen .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2006, 111 (D14)