Analysis of the temporal evolution of atmospheric Be-7 as a vector of the behavior of other radionuclides in the atmosphere

被引:41
作者
Baeza, A
DelRio, LM
Jimenez, A
Miro, C
Paniagua, JM
Rufo, M
机构
[1] Departamento de Física, F. Veterinaria-E. Politécnica, Universidad de Extremadura, 10071-Cáceres, Avda. de la Universidad s/n
来源
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY-ARTICLES | 1996年 / 207卷 / 02期
关键词
D O I
10.1007/BF02071239
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
The mean weekly levels of Be-7 in the atmosphere of Caceres (Spain) was measured for three consecutive years, from 1992 to 1994. The values showed a strongly seasonal behavior, conditioned fundamentally by two effects: (1) the incorporation of Be-7 into the low layers of the troposphere due to the displacement of masses of air from higher layers caused by the solar irradiation, and (2) the washing of Be-7 out of the atmosphere by rain. From the quantification of these two effects, the residence time of Be-7 was determined in die atmosphere at ground level as 10.3 days, with an interval for the standard error of 9.0 and 12.1 days. Modelling the temporal evolution of this radionuclide we were able to explain 90.72% of the variance of the measured activity levels. Using the effective residence time of Be-7, we were able to justify the diversity of values obtained for the deposition of Cs-137 in different soils of the province of Caceres due to the fallout from atmospheric nuclear blasts.
引用
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页码:331 / 344
页数:14
相关论文
共 17 条
[1]  
ANAND SJS, 1988, P ATM AER NUCL BERL
[2]  
[Anonymous], 1993, SOURC EFF ION RAD
[3]   BACKGROUND LEVELS OF ATMOSPHERIC DEPOSITION TO GROUND AND TEMPORAL VARIATION OF I-129, I-127, CS-137 AND BE-7 IN A RURAL AREA OF GERMANY [J].
BACHHUBER, H ;
BUNZL, K .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 1992, 16 (01) :77-89
[4]   SURFACE AND DEPTH FALLOUT DISTRIBUTION OF CS-137 AND SR-90 IN SOILS OF CACERES (SPAIN) - DOSE COMMITMENTS DUE TO EXTERNAL IRRADIATION [J].
BAEZA, A ;
DELRIO, M ;
MIRO, C ;
PANIAGUA, J .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY-LETTERS, 1993, 175 (04) :297-316
[5]  
BAEZA A, 1993, APPL RADIAT ISOTOPES, V43, P833
[6]   PRELIMINARY INVESTIGATIONS ON BE-7 AS A TRACER IN THE STUDY OF ENVIRONMENTAL PROCESSES [J].
BETTOLI, MG ;
CANTELLI, L ;
DEGETTO, S ;
TOSITTI, L ;
TUBERTINI, O ;
VALCHER, S .
JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY-ARTICLES, 1995, 190 (01) :137-147
[7]   FACTORS THAT CAUSE SEASONAL-VARIATIONS IN BERYLLIUM-7 CONCENTRATIONS IN SURFACE AIR [J].
FEELY, HW ;
LARSEN, RJ ;
SANDERSON, CG .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 1989, 9 (03) :223-249
[8]  
Hewit C.N., 1992, METHODS ENV DATA ANA
[9]   PRECIPITATION SCAVENGING STUDIES OF RADIONUCLIDES IN AIR USING COSMOGENIC BE-7 [J].
ISHIKAWA, Y ;
MURAKAMI, H ;
SEKINE, T ;
YOSHIHARA, K .
JOURNAL OF ENVIRONMENTAL RADIOACTIVITY, 1995, 26 (01) :19-36
[10]  
Kathren R. L., 1984, RADIOACTIVITY ENV SO