Low-temperature anomalies in strong and fragile glass formers

被引:148
作者
Sokolov, AP
Calemczuk, R
Salce, B
Kisliuk, A
Quitmann, D
Duval, E
机构
[1] CEA,SPSMS,LCP,F-38054 GRENOBLE 9,FRANCE
[2] FREE UNIV BERLIN,INST PHYS EXPT,D-14195 BERLIN,GERMANY
[3] UNIV LYON 1,LAB PHYSICOCHIM MAT LUMINESCENTS,LYON,FRANCE
关键词
D O I
10.1103/PhysRevLett.78.2405
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The low-temperature anomalies of glass forming systems are analyzed focusing on the concept of fragility. It is shown that two extremes on the fragility plot, SiO2 and Ca0.4K0.6(NO3)(1.4), show a strong difference in specific heat in the range of excess vibrational contribution. This difference cannot be explained in the framework of the soft potential model in its present state. A relation between the excess vibrational contribution and the amount of structural fluctuations is suggested. It is shown that the suggested relation explains the found difference in low-temperature specific heat between strong and fragile glass formers.
引用
收藏
页码:2405 / 2408
页数:4
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