Construction of Conjugated Carbon Nitride Nanoarchitectures in Solution at Low Temperatures for Photoredox Catalysis

被引:571
作者
Cui, Yanjuan [1 ,2 ]
Ding, Zhengxin [1 ,2 ]
Fu, Xianzhi [1 ,2 ]
Wang, Xinchen [1 ,2 ]
机构
[1] Fuzhou Univ, Res Inst Photocatalysis, Fujian Prov Key Lab Photocatalysis, State Key Lab Breeding Base, Fuzhou 350002, Peoples R China
[2] Fuzhou Univ, Coll Chem & Chem Engn, Fuzhou 350002, Peoples R China
基金
中国国家自然科学基金;
关键词
carbon nitride; nanostructures; photocatalysis; solution processing; water splitting; SOLID-STATE NMR; IONOTHERMAL SYNTHESIS; HYDROGEN EVOLUTION; GRAPHITIC FORM; ROUTE; SEMICONDUCTORS; C3N4; CRYSTALLINE;
D O I
10.1002/anie.201206534
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Hot: Conjugated carbon nitride polymers (LCNs) are synthesized by hot-fluid annealing in one pot. The LCNs possess a narrow band gap, have a complex nanostructure, and show enhanced photochemical performances. The described synthesis approach will allow the rational creation of a wide variety of polymeric carbon nitride semiconductors at low temperature in solutions, with control of structural complexity, electronic structure, and surface functionality. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:11814 / 11818
页数:5
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