Self-consistent model for second-harmonic near-field microscopy

被引:39
作者
Bozhevolnyi, SI
Lozovski, VZ
机构
[1] Aalborg Univ, Inst Phys, DK-9220 Aalborg, Denmark
[2] NAS Ukraine, Inst Semicond Phys, UA-252022 Kiev, Ukraine
关键词
D O I
10.1103/PhysRevB.61.11139
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
A macroscopic self-consistent approach that allows one to describe image formation rigorously in second-harmonic (SH) scanning near-field optical microscopy is developed. The SH held is determined by taking consistently into account both the linear and nonlinear contributions in the effective current, i.e., the currents generated by the self-consistent fields at the fundamental frequency (FF) and SH frequency. The self-consistent problem for both frequencies is solved exactly with a new approach to the determination of the Green dyadic of the system. General expressions for the FF and SH fields are obtained in terms of the effective susceptibility of the probe-object system. Image formation in the illumination SH near-field microscopy is considered within the framework of the approach developed. Near-field optical FF and SH images are calculated for different polarization configurations and parameters of a rectangular object with nonlinear susceptibility We show that the polarization selection rules used in conventional (far-field) SH experiments cannot be applied for SH near-field microscopy and that the SH signal detected in the forbidden polarization configurations may become comparable with the signal in the allowed configurations.
引用
收藏
页码:11139 / 11150
页数:12
相关论文
共 30 条
  • [1] Abrikosov A. A., 1965, QUANTUM FIELD THEORE, V2nd
  • [2] Near-field nonlinear optical spectroscopy of Langmuir-Blodgett films
    Bozhevolnyi, SI
    Geisler, T
    [J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA A-OPTICS IMAGE SCIENCE AND VISION, 1998, 15 (08): : 2156 - 2162
  • [3] Near-field optical microscopy of nonlinear susceptibilities
    Bozhevolnyi, SI
    Vohnsen, B
    Pedersen, K
    [J]. OPTICS COMMUNICATIONS, 1998, 150 (1-6) : 49 - 55
  • [4] Bozhevolnyi SI, 1999, PHYS STATUS SOLIDI A, V175, P331, DOI 10.1002/(SICI)1521-396X(199909)175:1<331::AID-PSSA331>3.0.CO
  • [5] 2-1
  • [6] Far- and near-field second-harmonic imaging of ferroelectric domain walls
    Bozhevolnyi, SI
    Pedersen, K
    Skettrup, T
    Zhang, XS
    Belmonte, M
    [J]. OPTICS COMMUNICATIONS, 1998, 152 (4-6) : 221 - 224
  • [7] CONTROL OF THE TIP SURFACE DISTANCE IN NEAR-FIELD OPTICAL MICROSCOPY
    BOZHEVOLNYI, SI
    KELLER, O
    XIAO, M
    [J]. APPLIED OPTICS, 1993, 32 (25): : 4864 - 4868
  • [8] CHEN KM, 1977, P IEEE, V65, P1202
  • [9] Near-field optics theories
    Girard, C
    Dereux, A
    [J]. REPORTS ON PROGRESS IN PHYSICS, 1996, 59 (05) : 657 - 699
  • [10] GENERATION OF OPTICAL STANDING WAVES AROUND MESOSCOPIC SURFACE-STRUCTURES - SCATTERING AND LIGHT CONFINEMENT
    GIRARD, C
    DEREUX, A
    MARTIN, OJF
    DEVEL, M
    [J]. PHYSICAL REVIEW B, 1995, 52 (04): : 2889 - 2898