Floating double probe characteristics of non-thermal plasmas in the presence of zeolite

被引:47
作者
Liu, CJ [1 ]
Wang, JX
Yu, KL
Eliasson, B
Xia, Q
Xue, BZ
Zhang, YH
机构
[1] Tianjin Univ, State Key Lab C1 Chem Technol, Tianjin 300072, Peoples R China
[2] Tianjin Univ, ABB Plasma Greenhouse Gas Chem Lab, Tianjin 300072, Peoples R China
[3] Tianjin Univ, Dept Appl Phys, Tianjin 300072, Peoples R China
[4] ABB Corp Res Ltd, CH-5405 Baden, Switzerland
基金
中国国家自然科学基金;
关键词
non-thermal plasma; glow discharge; double-probe characteristic; zeolite; plasma chemical processing; Langmuir probe;
D O I
10.1016/S0304-3886(01)00173-5
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
The combination of catalyst and non-thermal plasmas has led to some unusual chemical behaviors, especially with zeolite catalyst. A mechanism has been proposed to explain the observed interaction between catalyst and non-thermal plasmas. This mechanism includes two aspects: plasma promoted or induced catalysis and catalyst enhanced non-equilibrium of nonthermal plasmas. In this paper, we present some direct experimental evidence for the catalyst (zeolite)-enhanced non-equilibrium of non-thermal plasmas suggesting the use of zeolite increases, significantly, the electron temperature of non-thermal plasmas, while the gas temperature remains unchanged. A floating double-probe characteristic has been utilized to measure the electron temperature. Compared to the case without zeolite, the electron temperature of non-thermal plasmas with Mo-Zn/HZSM-5 increases up to 250%, while, at the same time, the discharge power reduces 58%, compared to that without zeolite. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:149 / 158
页数:10
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