Controlling pore size distributions of MCM-41 by direct synthesis

被引:49
作者
Wu, CN [1 ]
Tsai, TS [1 ]
Liao, CN [1 ]
Chao, KJ [1 ]
机构
[1] TSING HUA UNIV,DEPT CHEM,HSINCHU,TAIWAN
来源
MICROPOROUS MATERIALS | 1996年 / 7卷 / 04期
关键词
MCM-41; zeolite; mesoporous materials; N-2 adsorption isotherm; electron microscope; pore size distribution; MESOPOROUS MOLECULAR-SIEVES; PHYSISORPTION; ADSORPTION; ADSORBENT; NITROGEN; OXYGEN; ZSM-5;
D O I
10.1016/0927-6513(96)00049-1
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
A series of silicate, aluminosilicate, titanosilicate and vanadosilicate MCM-41 zeolites consisting of binodal pore systems of mesopore/macropore and mesopore only were synthesized under various conditions. The N-2 adsorption-desorption isotherm and electron-microscope investigations indicate that the pore size distribution is controlled by water content and by the silica source in reactant mixtures.
引用
收藏
页码:173 / 185
页数:13
相关论文
共 45 条
[1]   HIGH-RESOLUTION TRANSMISSION ELECTRON-MICROSCOPY OF MESOPOROUS MCM-41 TYPE MATERIALS [J].
ALFREDSSON, V ;
KEUNG, M ;
MONNIER, A ;
STUCKY, GD ;
UNGER, KK ;
SCHUTH, F .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1994, (08) :921-922
[2]   THE DETERMINATION OF PORE VOLUME AND AREA DISTRIBUTIONS IN POROUS SUBSTANCES .1. COMPUTATIONS FROM NITROGEN ISOTHERMS [J].
BARRETT, EP ;
JOYNER, LG ;
HALENDA, PP .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1951, 73 (01) :373-380
[3]   A NEW FAMILY OF MESOPOROUS MOLECULAR-SIEVES PREPARED WITH LIQUID-CRYSTAL TEMPLATES [J].
BECK, JS ;
VARTULI, JC ;
ROTH, WJ ;
LEONOWICZ, ME ;
KRESGE, CT ;
SCHMITT, KD ;
CHU, CTW ;
OLSON, DH ;
SHEPPARD, EW ;
MCCULLEN, SB ;
HIGGINS, JB ;
SCHLENKER, JL .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1992, 114 (27) :10834-10843
[4]  
BHORE NA, 1992, Patent No. 5134243
[5]   PHYSISORPTION OF NITROGEN AND OXYGEN BY MCM-41, A MODEL MESOPOROUS ADSORBENT [J].
BRANTON, PJ ;
HALL, PG ;
SING, KSW .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1993, (16) :1257-1258
[6]   PHYSISORPTION OF ARGON, NITROGEN AND OXYGEN BY MCM-41, A MODEL MESOPOROUS ADSORBENT [J].
BRANTON, PJ ;
HALL, PG ;
SING, KSW ;
REICHERT, H ;
SCHUTH, F ;
UNGER, KK .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1994, 90 (19) :2965-2967
[7]  
CASCI JL, 1994, STUD SURF SCI CATAL, V85, P329
[8]  
CHAO K, IN PRESS
[9]   KINETIC-STUDIES ON THE FORMATION OF ZEOLITE ZSM-5 [J].
CHAO, KJ ;
TASI, TC ;
CHEN, MS ;
WANG, I .
JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS I, 1981, 77 :547-555
[10]   STUDIES ON MESOPOROUS MATERIALS .1. SYNTHESIS AND CHARACTERIZATION OF MCM-41 [J].
CHEN, CY ;
LI, HX ;
DAVIS, ME .
MICROPOROUS MATERIALS, 1993, 2 (01) :17-26