Charge-orbital ordering and verwey transition in magnetite measured by resonant soft X-ray scattering

被引:93
作者
Huang, DJ [1 ]
Lin, HJ
Okamoto, J
Chao, KS
Jeng, HT
Guo, GY
Hsu, CH
Huang, CM
Ling, DC
Wu, WB
Yang, CS
Chen, CT
机构
[1] Natl Synchrotron Radiat Res Ctr, Hsinchu 30076, Taiwan
[2] Natl Chiao Tung Univ, Dept Electrophys, Hsinchu 30010, Taiwan
[3] Natl Ctr Theoret Sci, Div Phys, Hinchu 30013, Taiwan
[4] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan
[5] Tamkang Univ, Dept Phys, Tamsui 25137, Taiwan
关键词
D O I
10.1103/PhysRevLett.96.096401
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report experimental evidence for the charge-orbital ordering in magnetite below the Verwey transition temperature T-V. Measurements of O K-edge resonant x-ray scattering on magnetite reveal that the O 2p states in the vicinity of the Fermi level exhibit a charge-orbital ordering along the c axis with a spatial periodicity of the doubled lattice parameter of the undistorted cubic phase. Such a charge-orbital ordering vanishes abruptly above T-V and exhibits a thermal hysteresis, correlating closely with the Verwey transition in magnetite.
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页数:4
相关论文
共 26 条
[1]   Crystallization of charge holes in the spin ladder of Sr14Cu24O41 [J].
Abbamonte, P ;
Blumberg, G ;
Rusydi, A ;
Gozar, A ;
Evans, PG ;
Siegrist, T ;
Venema, L ;
Eisaki, H ;
Isaacs, ED ;
Sawatzky, GA .
NATURE, 2004, 431 (7012) :1078-1081
[2]   A structural probe of the doped holes in cuprate superconductors [J].
Abbamonte, P ;
Venema, L ;
Rusydi, A ;
Sawatzky, GA ;
Logvenov, G ;
Bozovic, I .
SCIENCE, 2002, 297 (5581) :581-584
[3]   Orbital ordering, Jahn-Teller distortion, and resonant x-ray scattering in KCuF3 -: art. no. 085117 [J].
Binggeli, N ;
Altarelli, M .
PHYSICAL REVIEW B, 2004, 70 (08) :085117-1
[4]   HIGH-RESOLUTION PHOTOEMISSION SPECTROSCOPY OF THE VERWEY TRANSITION IN FE3O4 [J].
CHAINANI, A ;
YOKOYA, T ;
MORIMOTO, T ;
TAKAHASHI, T ;
TODO, S .
PHYSICAL REVIEW B, 1995, 51 (24) :17976-17979
[5]   Resonant "forbidden" reflections in magnetite [J].
García, J ;
Subías, G ;
Proietti, MG ;
Renevier, H ;
Joly, Y ;
Hodeau, JL ;
Blasco, J ;
Sánchez, MC ;
Bérar, JF .
PHYSICAL REVIEW LETTERS, 2000, 85 (03) :578-581
[6]   The Verwey transition -: a new perspective [J].
García, J ;
Subias, G .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2004, 16 (07) :R145-R178
[7]   Absence of charge ordering below the Verwey transition temperature in magnetite -: art. no. 054110 [J].
García, J ;
Subías, G ;
Proietti, MG ;
Blasco, J ;
Renevier, H ;
Hodeau, JL ;
Joly, Y .
PHYSICAL REVIEW B, 2001, 63 (05)
[8]  
GUO G, UNPUB
[9]   Metal-insulator transitions [J].
Imada, M ;
Fujimori, A ;
Tokura, Y .
REVIEWS OF MODERN PHYSICS, 1998, 70 (04) :1039-1263
[10]   Charge-orbital ordering and verwey transition in magnetite [J].
Jeng, HT ;
Guo, GY ;
Huang, DJ .
PHYSICAL REVIEW LETTERS, 2004, 93 (15) :156403-1