Three-dimensional coherent x-ray diffraction imaging of a ceramic nanofoam: Determination of structural deformation mechanisms

被引:79
作者
Barty, A. [1 ]
Marchesini, S. [1 ,2 ,3 ]
Chapman, H. N. [1 ,3 ]
Cui, C. [2 ]
Howells, M. R. [2 ]
Shapiro, D. A. [2 ]
Minor, A. M. [2 ]
Spence, J. C. H. [4 ]
Weierstall, U. [4 ]
Ilavsky, J. [5 ]
Noy, A. [1 ]
Hau-Riege, S. P. [1 ]
Artyukhin, A. B. [1 ]
Baumann, T. [1 ]
Willey, T. [1 ]
Stolken, J. [1 ]
van Buuren, T. [1 ]
Kinney, J. H. [6 ]
机构
[1] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA
[2] Univ Calif Berkeley, Lawrence Berkeley Lab, Berkeley, CA 94720 USA
[3] Univ Calif Davis, Ctr Biophoton Sci & Technol, Sacramento, CA 95817 USA
[4] Arizona State Univ, Dept Phys & Astron, Tempe, AZ 85287 USA
[5] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
[6] Univ Calif San Francisco, Dept Prevent & Restorat Dent Sci, San Francisco, CA 94143 USA
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.101.055501
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Ultralow density polymers, metals, and ceramic nanofoams are valued for their high strength-to-weight ratio, high surface area, and insulating properties ascribed to their structural geometry. We obtain the labrynthine internal structure of a tantalum oxide nanofoam by x-ray diffractive imaging. Finite-element analysis from the structure reveals mechanical properties consistent with bulk samples and with a diffusion-limited cluster aggregation model, while excess mass on the nodes discounts the dangling fragments hypothesis of percolation theory.
引用
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页数:4
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