Catalytic investigation of Fe-ZSM5 in the selective catalytic reduction of NOx with NH3

被引：38

作者：

Devadas, M ^{[1
]}

Kröcher, O ^{[1
]}

Wokaun, A ^{[1
]}

机构：

[1] Paul Scherrer Inst, CH-5232 Villigen, Switzerland

来源：

REACTION KINETICS AND CATALYSIS LETTERS | 2005年 / 86卷 / 02期

关键词：

Fe-ZSM5; DeNOx; monolith; SCR; selective catalytic reduction; ammonia;

D O I：

10.1007/s11144-005-0331-1

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Fe-ZSM5 coated on a cordierite monolith was characterized and tested in the selective reduction of nitrogen oxides (NOx) with ammonia. More than 70% of the NO, were converted at T >= 350 degrees C if only NO was present in the feed. For equimolar amounts of NO and NO2 in the feed, NOx conversions of over 90% were reached for T = 200-450 degrees C. Hydrothermal ageing of Fe-ZSM5 resulted in a small loss in NOx conversion and enhanced N2O formation.

引用

页码：347 / 354

页数：8

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